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51.
Search for Anisotropy in the Ultra High Energy Cosmic Ray Spectrum using the Telescope Array Surface Detector
R.U. Abbasi, Jon Paul Lundquist, 2017, other component parts

Abstract: The Telescope Array (TA) experiment is located in the western desert of Utah, USA, and observes ultra high energy cosmic rays (UHECRs) in the Northern hemisphere. At the highest energies, E>10~EeV, the shape of cosmic ray energy spectrum may carry an imprint of the source density distribution along the line of sight different in different directions of the sky. In this study, we search for such directional variations in the shape of the energy spectrum using events observed with the Telescope Array's surface detector. We divide the TA field of view into two nearly equal-exposure regions: the "on-source" region which we define as ±30∘ of the supergalactic plane containing mostly nearby structures, and the complementary "off-source" region where the sources are further away on average. We compare the UHECR spectra in these regions by fitting them to the broken power law and comparing the resulting parameters. We find that the off-source spectrum has an earlier break at highest energies. The chance probability to obtain such or larger difference in statistically equivalent distributions is estimated as 6.2±1.1×10−4 (3.2σ) by a Monte-Carlo simulation. The observed difference in spectra is in a reasonable quantitative agreement with a simplified model that assumes that the UHECR sources trace the galaxy distribution from the 2MRS catalogue, primary particles are protons and the magnetic deflections can be neglected.
Keywords: cosmic radiation: UHE, detector: surface, cosmic radiation: spectrum, cosmic radiation: energy spectrum, deflection: magnetic, numerical calculations: Monte Carlo, anisotropy
Published in RUNG: 27.04.2020; Views: 2744; Downloads: 98
.pdf Full text (169,05 KB)

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Magnetic anisotropy of strontium ferrite nanoparticles
Cesar de Julian Fernandez, D. Mishra, M. Cabassi, M. Petrecca, M. Albino, M. Suara-Muzquiz, Petra Jenuš, A. Quesada, T. Schliesch, Blaž Belec, C. Sangregorio, F. Albertini, 2019, published scientific conference contribution abstract

Keywords: hexaferrite, nanoparticles, magnetic anisotropy, SPD
Published in RUNG: 04.06.2019; Views: 3468; Downloads: 0
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Synthesis of inorganic anisotropic nanoparticles
Blaž Belec, invited lecture at foreign university

Keywords: Magnetic nanoparticles, anisotropic nanoparticles, exchange coupled nanoparticles
Published in RUNG: 10.04.2019; Views: 3261; Downloads: 0
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57.
Combining hard and soft magnetic phases by mechanical mixing
Blaž Belec, Cesar De Jilian Fernandez, Daniela Bertoni, other performed works

Keywords: Magnetic materials Magnetodipolar interactions lorenz microscopy
Published in RUNG: 12.02.2019; Views: 3335; Downloads: 0
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58.
Seminar on Bimagnetic Composites
Blaž Belec, other monographs and other completed works

Keywords: BI-MAGNETIC composites nanoparticles
Published in RUNG: 09.01.2019; Views: 4102; Downloads: 115
URL Link to full text

59.
Synthesis and characterization of inorganic anisotropic nanoparticles
Belec Blaž, invited lecture at foreign university

Keywords: Nanoparticles anisotropic particles magnetic nanocompoistes topological insulator
Published in RUNG: 05.11.2018; Views: 3362; Downloads: 0
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60.
PHOTO-EXCITATION ENERGY INFLUENCE ON THE PHOTOCONDUCTIVITY OF ORGANIC SEMICONDUCTORS
Nadiia Pastukhova, 2018, doctoral dissertation

Abstract: In this work, we experimentally studied the influence of photoexcitation energy influence on the charge transport in organic semiconductors. Organic semiconductors were small molecules like corannulene, perylene and pentacene derivatives, polymers such as polythiophene and benzothiophene derivatives, and graphene, along with combinations of these materials in heterojunctions or composites. The first part of this study is focused on the photoexcitation energy influence on the transient photoconductivity of non-crystalline curved π-conjugated corannulene layers. The enhanced photoconductivity, in the energy range where optical absorption is absent, is deduced from theoretical predictions of corannulene gas-phase excited state spectra. Theoretical analysis reveals a consistent contribution involving transitions to Super Atomic Molecular Orbitals (SAMOs), a unique set of diffuse orbitals typical of curved π-conjugated molecules. More, the photoconductivity of the curved corannulene was compared to the π-conjugated planar N,N′-1H,1H- perfluorobutyldicyanoperylene-carboxydi-imide (PDIF-CN2), where the photoexcitation energy dependence of photocurrent closely follows the optical absorption spectrum. We next characterized charge transport in poly(3-hexylthiophene) (P3HT) layers deposited from solution. Our results indicate that time-of-flight (TOF) mobility depends on the photoexcitation energy. It is 0.4× 10 −3 cm 2 /Vs at 2.3 eV (530 nm) and doubles at 4.8 eV (260 nm). TOF mobility was compared to field-effect (FET) mobility of P3HT field-effect transistors (OFETs). The FET mobility was similar to the 2.3 eV excitation TOF mobility. In order to improve charge mobility, graphene nanoparticles were blended within a P3HT solution before the deposition. We found that the mobility significantly improves upon the addition of graphene nanoparticles of a weight ratio as low as 0.2 %. FET mobility increases with graphene concentration up to a value of 2.3× 10 −2 cm 2 /Vs at 3.2 %. The results demonstrate that phase segregation starts to influence charge transport at graphene concentration of 0.8 % and above. Hence, the graphene cannot form a bridged conduction channel between electrodes, which would cancel the semiconducting effect of the polymer composite. An alternative approach to enhance mobility is to optimize the molecular ordering of organic semiconductors. For that purpose, we studied an innovative nanomesh device. Free-standing nanomesh devices were used to form nanojunctions of N,N′- iiDioctyl-3,4,9,10-perylenedicarboximide (PTCDI-C8) nanowires and crystalline bis(triisopropylsilylethinyl)pentacene (TIPS-PEN). We characterized the photocurrent response time of this novel nanomesh scaffold device. The photoresponse time depends on the photon energy. It is between 4.5 − 5.6 ns at 500 nm excitation wavelength and between 6.7 − 7.7 ns at 700 nm excitation wavelength. In addition, we found that thermal annealing reduces charge carrier trapping in crystalline nanowires. This confirms that the structural defects are crucial to obtaining high photon-to-charge conversion efficiency and subsequent transport from pn junction in heterostructured materials. Structural defects also influence the power conversion efficiency of organic heterostructured photovoltaics (OPVs). Anticipating that polymers with different backbone lengths produce different level of structural defects, we examined charge transport dependence on the molecular weight of poly[4,8-bis(5-(2- ethylhexyl)thiophen-2-yl)benzo[1,2-b;4,5-b']dithiophene-2,6-diyl-alt-(4-(2- ethylhexyl)-3-fluorothieno[3,4-b]thiophene-)-2-carboxylate-2-6-diyl] (PTB7-Th) from 50 kDa to 300 kDa. We found p-type hopping transport in PTB7-Th, characterized by 0.1 – 3× 10 −2 cm 2 /Vs mobility, which increases with temperature and electric field. The polymer molecular weight exhibits a non-trivial influence on charge transport. FET mobility in the saturation regime increases with molecular weight. A similar trend is observed in TOF mobility and FET mobility in the linear regime, except for the 100kDa polymer, which manifests in the highest mobility due to reduced charge trapping. The lowest trapping at the dielectric interface of OFET is observed at 200 kDa. In addition, the 200 kDa polymer exhibits the lowest activation energy of the charge transport. Although the 100 kDa polymer indicates the highest mobility, OPVs using the 200 kDa polymer exhibit the best performance in terms of power conversion efficiency.
Keywords: organic semiconductors, optical absorption spectroscopy, time-of-flight photoconductivity, transient photocurrent spectroscopy, organic thin film transistors, atomic force microscopy, superatomic molecular orbitals, pn heterojunction, organic nanowires, graphene, composites, charge mobility, charge trapping, temperature dependence, photodetector, photovoltaic, solar cell, organic electronics
Published in RUNG: 08.10.2018; Views: 5389; Downloads: 163
.pdf Full text (4,56 MB)

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