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Abstract: The aim of the dissertation was to study aerosol loading distributions and properties over the Vipava valley, a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin. An infrared Mie and a two-wavelength polarization Raman lidar systems were used as main detection tools. The polarization Raman lidar, which provides the capability to extract the extinction coefficient, backscatter coefficients, depolarization ratio, backscatter Ångström exponent, lidar ratio and water vapor mixing ratio profiles, was itself designed, built and calibrated as a part of this thesis. Lidar data, combined with in-situ measurements, was used to determine detailed information on different aerosol types. Vertical profiles of aerosol mass concentration were extracted from the Mie lidar data taken in April 2016, where the in-situ measurements of aerosol size distribution and number concentration as well as aerosol absorption coefficient and black carbon mass concentration were used to estimate the mass extinction efficiency (MEE). Aerosol morphology and chemical composition determined by SEM-EDX on sampled particles were used for the identification of primary aerosol types. Two cases with different atmospheric conditions (long range mineral dust transport and local biomass burning) and different expected the dominant presence of specific aerosol types (mineral dust and soot) were investigated in more detail. They revealed significantly different aerosol properties and distributions within the valley, affecting radiative heat exchange. A more detailed investigation of aerosol properties throughout the troposphere in different atmospheric conditions was made possible by the two-wavelength polarization Raman lidar system, deployed in Ajdovščina (town of Vipava valley) from September 2017. Using its aerosol identification capabilities, based on particle depolarization ratio and lidar ratio measurements, it was possible to identify predominant aerosol types in the observed atmospheric structures, for example in different atmospheric layers in the case of the stratified atmosphere. Primary anthropogenic aerosols within the valley were found to be mainly emitted from two sources: individual domestic heating systems, which mostly use biomass fuel and traffic. Natural aerosols, transported over large distances, such as mineral dust and sea salt, were observed both above and entering into the planetary boundary layer. Backscatter contribution of each aerosol type was separated and the corresponding extinction contribution was derived from lidar observations.
Found in: ključnih besedah
Summary of found: ...infrared Mie and a two-wavelength polarization Raman lidar systems were used as main detection tools. The...
Keywords: Vipava valley, aerosol distribution, aerosol characterization, lidar remote sensing, in-situ measurements, aerosol loading.
Published: 23.10.2018; Views: 3681; Downloads: 73
Fulltext (29,39 MB)

Abstract: Aerosol vertical profiles are valuable inputs for the evaluation of aerosol transport models, in order to improve the understanding of aerosol pollution ventilation processes which drive the dispersion of pollutants in mountainous regions. With the aim of providing high-accuracy vertical distributions of particle mass concentration for the study of aerosol dispersion in small-scale valleys, vertical profiles of aerosol mass concentration for aerosols from different sources (including Saharan dust and local biomass burning events) were investigated over the Vipava valley, Slovenia, a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin. The analysis was based on datasets taken between 1–30 April 2016. In-situ measurements of aerosol size, absorption, and mass concentration were combined with lidar remote sensing, where vertical profiles of aerosol concentration were retrieved. Aerosol samples were characterized by SEM-EDX, to obtain aerosol morphology and chemical composition. Two cases with expected dominant presence of different specific aerosol types (mineral dust and biomass-burning aerosols) show significantly different aerosol properties and distributions within the valley. In the mineral dust case, we observed a decrease of the elevated aerosol layer height and subsequent spreading of mineral dust within the valley, while in the biomass-burning case we observed the lifting of aerosols above the planetary boundary layer (PBL). All uncertainties of size and assumed optical properties, combined, amount to the total uncertainty of aerosol mass concentrations below 30% within the valley. We have also identified the most indicative in-situ parameters for identification of aerosol type.
Found in: ključnih besedah
Summary of found: ...absorption, and mass concentration were combined with lidar remote sensing, where vertical profiles of aerosol...
Keywords: valley air pollution, aerosol vertical distributions, lidar remote sensing, in-situ measurements, aerosol identification
Published: 09.01.2019; Views: 1362; Downloads: 46
Fulltext (7,43 MB)

Abstract: Vipava valley in Slovenia is a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin. Aerosol loading distributions and optical properties were investigated using a two-wavelength polarization Raman LiDAR, which provided extinction coefficient, backscatter coefficient, depolarization ratio, backscatter Ångström exponent and LiDAR ratio profiles. Two different representative meteorological situations were investigated to explore the possibility of identifying aerosol types present in the valley. In the first case, we investigated the effect of strong downslope (Bora) wind on aerosol structures and characteristics. In addition to observing Kelvin–Helmholtz instability above the valley, at the height of the adjacent mountain ridge, we found new evidence for Bora-induced processes which inject soil dust aerosols into the free troposphere up to twice the height of the planetary boundary layer (PBL). In the second case, we investigated aerosol properties and distributions in stable weather conditions. From the observed stratified vertical aerosol structure and specific optical properties of different layers we identified predominant aerosol types in these layers.
Found in: ključnih besedah
Keywords: aerosol structures, aerosol characterization, polarization Raman LiDAR, Vipava valley
Published: 08.03.2019; Views: 1191; Downloads: 51
Fulltext (3,11 MB)

Abstract: The Cherenkov Telescope Array (CTA) is the next generation ground-based observatory for gamma-ray astronomy at very-high energies. Employing more than 100 (north and south sites) Imaging Atmospheric Cherenkov Telescopes in the northern and southern hemispheres, it was designed to reach unprecedented sensitivity and energy resolution. Understanding and correcting for systematic biases on the absolute energy scale and instrument response functions will be a cru- cial issue for the performance of CTA. The Montpellier group and the Spanish/Italian/Slovenian collaboration are currently building two Raman LIDAR prototypes for the online atmospheric cal- ibration along the line-of-sight of the CTA. Requirements for such a solution include the ability to characterize aerosol extinction at two wavelengths to distances up to 30 km with an accuracy better than 5%, within exposure time scales of about a minute, steering capabilities and close interaction with the CTA array control and data acquisition system as well as other auxiliary in- struments. Our Raman LIDARs have design features that make them different from those used in atmospheric science and are characterized by large collecting mirrors (∼2.5 m 2 ), liquid light- guides that collect the light at the focal plane and transport it to the readout system, reduced acquisition time and highly precise Raman spectrometers. The Raman LIDARs will participate in a cross-calibration and characterization campaign of the atmosphere at the CTA North site at La Palma, together with other site characterization instruments. After a one-year test period there, an in-depth evaluation of the solutions adopted by the two projects will lead to a final Raman LIDAR design proposal for both CTA sites.
Found in: ključnih besedah
Summary of found: ...the Spanish/Italian/Slovenian collaboration are currently building two Raman LIDAR prototypes for the online atmospheric cal- ibration along...
Keywords: Raman lidar atmospheric calibration Cherenkov Telescope Array
Published: 29.08.2019; Views: 780; Downloads: 35
Fulltext (1,29 MB)

Abstract: We report on the design, construction and performance of a polarization Raman lidar, built for atmospheric monitoring in the Vipava valley in SW Slovenia, a regional air pollution hot-spot where aerosols are expected to originate from a number of different sources. Its key features are automatized remote operation capability and indoor deployment, which provide high duty cycle in all weather conditions. System optimization and performance studies include the calibration of the depolarization ratio, merging of near-range (analog) and far-range (photon-counting) data, determination of overlap functions and validation of the retrieved observables with radiosonde data.
Found in: ključnih besedah
Keywords: polarization Ramal lidar, Vipava valley, atmospheric monitoring
Published: 08.07.2020; Views: 404; Downloads: 0
Fulltext (3,88 MB)