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Naslov:Uranium bearing dissolved organic matter in the porewaters of uranium contaminated lake sediments
Avtorji:ID Novotnik, Breda, School of the Environment, Trent University, Peterborough, Ontario, Canada (Avtor)
ID Chen, Wei, Chemistry and Biochemistry Department, Wilfrid Laurier University, Waterloo, Ontario, Canada (Avtor)
ID Evans, R. Douglas, School of the Environment, Trent University, Peterborough, Ontario, Canada (Avtor)
Datoteke: Gradivo nima datotek, ki so prostodostopne za javnost. Gradivo je morda fizično dosegljivo v knjižnici fakultete, zalogo lahko preverite v COBISS-u. Povezava se odpre v novem oknu
Jezik:Angleški jezik
Vrsta gradiva:Delo ni kategorizirano
Tipologija:1.01 - Izvirni znanstveni članek
Organizacija:UNG - Univerza v Novi Gorici
Opis:Uranium (U) mobility in the environment strongly depends on its oxidation state and the presence of complexing agents such as inorganic carbon, phosphates, and dissolved organic matter (DOM). Despite the importance of DOM in U mobility, the exact mechanism is still poorly understood. Therefore, the aim of our investigation was to characterise sediment porewater DOM in two lakes in Ontario, Canada (Bow and Bentley Lakes) that were historically contaminated with U and propose possible composition of UO2-bearing DOM. Depth profiles of U concentrations in porewaters and total sediment digests reveal U levels of up to 1.3 mg L−1 in porewater and up to 0.8 mg−1 g in sediment. Depth profiles of U did not correlate with Fe, Mn, SO4 2−, or Eh profiles. Therefore, porewater DOM was analysed and taken into consideration as the primary source of U mobility. Porewater DOM in each sediment section (1 cm sections, 20 cm core length) was analysed by high-resolution electrospray ionisation mass spectrometry. PCA analyses of porewater DOM mass spectra showed grouping and clear separation of DOM in sediment sections with elevated U concentrations in comparison to sections with background U concentrations. Several criteria were set to characterise UO2-bearing DOM and more than 70 different molecules were found. The vast majority of these UO2-DOM compounds fell in the category of carboxyl-containing aliphatic molecules (H/C between 0.85 and 1.2 and O/C≤0.4) and had a mean value of m/z about 720.
Ključne besede:Uranium Lake sediments Porewater Disolved organic matter High resolution mass spectrometry
Verzija publikacije:Objavljena publikacija
Leto izida:2018
Št. strani:36-44
Številčenje:2018, 91
PID:20.500.12556/RUNG-4776-198dd4c5-11aa-ea38-3b64-ff8bd2ceeb94 Novo okno
COBISS.SI-ID:5460731 Novo okno
DOI:https://doi.org/10.1016/j.apgeochem.2018.01.009 Novo okno
NUK URN:URN:SI:UNG:REP:RIULFLNY
Datum objave v RUNG:09.10.2019
Število ogledov:4493
Število prenosov:0
Metapodatki:XML DC-XML DC-RDF
:
NOVOTNIK, Breda, CHEN, Wei in EVANS, R. Douglas, 2018, Uranium bearing dissolved organic matter in the porewaters of uranium contaminated lake sediments. Applied Geochemistry [na spletu]. 2018. Vol. 2018, no. 91, p. 36–44. [Dostopano 14 april 2025]. DOI https://doi.org/10.1016/j.apgeochem.2018.01.009. Pridobljeno s: https://repozitorij.ung.si/IzpisGradiva.php?lang=slv&id=4776
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Gradivo je del revije

Naslov:Applied Geochemistry
Leto izida:2018

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