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Naslov:Consistent determination of the heating rate of light-absorbing aerosol using wavelength- and time-dependent Aethalometer multiple-scattering correction
Avtorji:ID Ferrero, Luca (Avtor)
ID Bernardoni, Vera (Avtor)
ID Santagostini, Luca (Avtor)
ID Cogliati, Sergio (Avtor)
ID Soldan, Francesca (Avtor)
ID Valentini, Sara (Avtor)
ID Massabò, Dario (Avtor)
ID Močnik, Griša (Avtor)
ID Gregorič, Asta (Avtor)
ID Rigler, Martin (Avtor), et al.
Datoteke: Gradivo nima datotek, ki so prostodostopne za javnost. Gradivo je morda fizično dosegljivo v knjižnici fakultete, zalogo lahko preverite v COBISS-u. Povezava se odpre v novem oknu
Jezik:Angleški jezik
Vrsta gradiva:Neznano
Tipologija:1.01 - Izvirni znanstveni članek
Organizacija:UNG - Univerza v Novi Gorici
Opis:Accurate and temporally consistent measurements of light absorbing aerosol (LAA) heating rate (HR) and of its source apportionment (fossil-fuel, FF; biomass-burning, BB) and speciation (black and brown Carbon; BC, BrC) are needed to evaluate LAA short-term climate forcing. For this purpose, wavelength- and time-dependent accurate LAA absorption coefficients are required. HR was experimentally determined and apportioned (sources/species) in the EMEP/ACTRIS/COLOSSAL-2018 winter campaign in Milan (urban-background site). Two Aethalometers (AE31/AE33) were installed together with a MAAP, CPC, OPC, a low volume sampler (PM2.5) and radiation instruments. AE31/AE33 multiple-scattering correction factors (C) were determined using two reference systems for the absorption coefficient: 1) 5-wavelength PP_UniMI with low time resolution (12 h, applied to PM2.5 samples); 2) timely-resolved MAAP data at a single wavelength. Using wavelength- and time-independent C values for the AE31 and AE33 obtained with the same reference device, the total HR showed a consistency (i.e. reproducibility) with average values comparable at 95% probability. However, if different reference devices/approaches are used, i.e. MAAP is chosen as reference instead of a PP_UniMI, the HR can be overestimated by 23-30% factor (by both AE31/AE33). This became more evident focusing on HR apportionment: AE33 data (corrected by a wavelength- and time-independent C) showed higher HRFF (+24±1%) and higher HRBC (+10±1%) than that of AE31. Conversely, HRBB and HRBrC were -28±1% and -29±1% lower for AE33 compared to AE31. These inconsistencies were overcome by introducing a wavelength-dependent Cλ for both AE31 and AE33, or using multi-wavelength apportionment methods, highlighting the need for further studies on the influence of wavelength corrections for HR determination. Finally, the temporally-resolved determination of C resulted in a diurnal cycle of the HR not statistically different whatever the source- speciation- apportionment used.
Ključne besede:climate change, heating rate, black carbon, light absorbing aerosols
Leto izida:2021
Št. strani:str. 1-65
Številčenje:Vol. , 2021
PID:20.500.12556/RUNG-6582 Novo okno
COBISS.SI-ID:66309379 Novo okno
UDK:53
ISSN pri članku:0048-9697
DOI:10.1016/j.scitotenv.2021.148277 Novo okno
NUK URN:URN:SI:UNG:REP:TYYUYOLO
Datum objave v RUNG:09.06.2021
Število ogledov:3420
Število prenosov:0
Metapodatki:XML DC-XML DC-RDF
:
FERRERO, Luca, BERNARDONI, Vera, SANTAGOSTINI, Luca, COGLIATI, Sergio, SOLDAN, Francesca, VALENTINI, Sara, MASSABÒ, Dario, MOČNIK, Griša, GREGORIČ, Asta in RIGLER, Martin, 2021, Consistent determination of the heating rate of light-absorbing aerosol using wavelength- and time-dependent Aethalometer multiple-scattering correction. Science of the total environment [na spletu]. 2021. No. 2021, p. 1–65. [Dostopano 11 april 2025]. DOI 10.1016/j.scitotenv.2021.148277. Pridobljeno s: https://repozitorij.ung.si/IzpisGradiva.php?lang=slv&id=6582
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Gradivo je del revije

Naslov:Science of the total environment
Skrajšan naslov:Sci. total environ.
Založnik:Elsevier
ISSN:0048-9697
COBISS.SI-ID:26369024 Novo okno

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