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Naslov:Crystallizing covalent organic frameworks from metal organic framework through chemical induced-phase engineering
Avtorji:ID Khayum Mohammed, Abdul (Avtor)
ID Gaber, Safa (Avtor)
ID Raya, Jesus (Avtor)
ID Škorjanc, Tina (Avtor)
ID Elmerhi, Nada (Avtor)
ID Stephen, Sasi (Avtor)
ID Pena-Sánchez, Pilar (Avtor)
ID Gándara, Felipe (Avtor)
ID Hinder, Steven (Avtor)
ID Baker, Mark A. (Avtor)
ID Polychronopoulou, Kyriaki (Avtor)
ID Shetty, Dinesh (Avtor)
Datoteke:URL https://www.nature.com/articles/s41598-023-46573-3
 
.pdf s41598-023-46573-3.pdf (3,64 MB)
MD5: 43250986A83C6994C1C51874FD645EA6
 
URL https://www.nature.com/articles/s41598-023-46573-3
 
Jezik:Angleški jezik
Vrsta gradiva:Neznano
Tipologija:1.01 - Izvirni znanstveni članek
Organizacija:UNG - Univerza v Novi Gorici
Opis:The ordered porous frameworks like MOFs and COFs are generally constructed using the monomers through distinctive metal-coordinated and covalent linkages. Meanwhile, the inter-structural transition between each class of these porous materials is an under-explored research area. However, such altered frameworks are expected to have exciting features compared to their pristine versions. Herein, we have demonstrated a chemical-induction phase-engineering strategy to transform a two dimensional conjugated Cu-based SA-MOF (Cu-Tp) into 2D-COFs (Cu-TpCOFs). The structural phase transition offered in-situ pore size engineering from 1.1 nm to 1.5–2.0 nm. Moreover, the Cu-TpCOFs showed uniform and low percentage-doped (~ 1–1.5%) metal distribution and improved crystallinity, porosity, and stability compared to the parent Cu-Tp MOF. The construction of a framework from another framework with new linkages opens interesting opportunities for phase-engineering.
Ključne besede:metal organic framework, covalent organic framework, phase engineering, chemical transformation, porous materials
Datum objave:01.01.2023
Leto izida:2023
Št. strani:str. 1-7
Številčenje:Vol. 13, article no. ǂ19443
PID:20.500.12556/RUNG-8621-0d201bce-5b61-5f43-f9ae-525909bf51b0 Novo okno
COBISS.SI-ID:171577091 Novo okno
UDK:54
ISSN pri članku:2045-2322
DOI:10.1038/s41598-023-46573-3 Novo okno
NUK URN:URN:SI:UNG:REP:BA8JVMRY
Datum objave v RUNG:10.11.2023
Število ogledov:3841
Število prenosov:7
Metapodatki:XML DC-XML DC-RDF
:
KHAYUM MOHAMMED, Abdul, GABER, Safa, RAYA, Jesus, ŠKORJANC, Tina, ELMERHI, Nada, STEPHEN, Sasi, PENA-SÁNCHEZ, Pilar, GÁNDARA, Felipe, HINDER, Steven, BAKER, Mark A., POLYCHRONOPOULOU, Kyriaki in SHETTY, Dinesh, 2023, Crystallizing covalent organic frameworks from metal organic framework through chemical induced-phase engineering. Scientific reports [na spletu]. 2023. Vol. 13, no. 19443, p. 1–7. [Dostopano 7 april 2025]. DOI 10.1038/s41598-023-46573-3. Pridobljeno s: https://repozitorij.ung.si/IzpisGradiva.php?lang=slv&id=8621
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Gradivo je del revije

Naslov:Scientific reports
Skrajšan naslov:Sci. rep.
Založnik:Nature Publishing Group
ISSN:2045-2322
COBISS.SI-ID:18727432 Novo okno

Licence

Licenca:CC BY 4.0, Creative Commons Priznanje avtorstva 4.0 Mednarodna
Povezava:http://creativecommons.org/licenses/by/4.0/deed.sl
Opis:To je standardna licenca Creative Commons, ki daje uporabnikom največ možnosti za nadaljnjo uporabo dela, pri čemer morajo navesti avtorja.

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