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Ključne besede: photothermal interferometer, aerosol light absorption coefficient
Objavljeno v RUNG: 14.01.2022; Ogledov: 1948; Prenosov: 28
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Ključne besede: mineral dust, optical absorption, virtual impactor
Objavljeno v RUNG: 22.11.2021; Ogledov: 2086; Prenosov: 0
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Ključne besede: mineral dust, concentration, aerosols, air quality
Objavljeno v RUNG: 17.11.2021; Ogledov: 1835; Prenosov: 12
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Opis: This paper complements the existing studies of Bora flow properties in the Vipava valley with the study of Bora turbulence in a lower region of the troposphere. The turbulence characteristics of Bora flow were derived from high resolution Doppler wind lidar measurements during eight Bora wind episodes that occurred in November and December 2019. Based on the vertical profiles of wind velocity, from 80 to 180 m above the valley floor, the turbulence intensity related to all three spatial directions and the along-wind integral length scales related to three velocity components were evaluated and compared to the approximations given in international standards. The resulting turbulence characteristics of Bora flow in a deep mountain valley exhibited interesting behaviour, differing from the one expected and suggested by standards. The intensity of turbulence during Bora episodes was found to be quite strong, especially regarding the expected values for that particular category of terrain. The specific relationship between along-wind, lateral and vertical intensity was evaluated as well. The scales of turbulence in the along-wind direction were found to vary widely between different Bora episodes and were rather different from the approximations given by standards, with the most significant deviations observed for the along-wind length scale of the vertical velocity component. Finally, the periodicity of flow structures above the valley was assessed, yielding a wide range of possible periods between 1 and 10 min, thus confirming some of the previous observations from the studies of Bora in the Vipava valley.
Ključne besede: doppler wind lidar, Bora wind, turbulence intensity, complex terrain, turbulence integral length scale
Objavljeno v RUNG: 05.11.2021; Ogledov: 2169; Prenosov: 42
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Opis: Providing reliable observations of aerosol particles' absorption properties at spatial and temporal resolutions suited to climate models is of utter importance to better understand the effects that atmospheric particles have on climate. Nowadays, one of the instruments most widely used in international monitoring networks for in situ surface measurements of light absorption properties of atmospheric aerosol particles is the multi-wavelength dual-spot Aethalometer, AE33. The AE33 derives the absorption coefficients of aerosol particles at seven different wavelengths from the measurements of the optical attenuation of light through a filter where particles are continuously collected. An accurate determination of the absorption coefficients from the AE33 instrument relies on the quantification of the non-linear processes related to the sample collection on the filter. The multiple-scattering correction factor (C), which depends on the filter tape used and on the optical properties of the collected particles, is the parameter with both the greatest uncertainty and the greatest impact on the absorption coefficients derived from the AE33 measurements. Here we present an in-depth analysis of the AE33 multiple-scattering correction factor C and its wavelength dependence for two different and widely used filter tapes, namely the old, and most referenced, TFE-coated glass, or M8020, filter tape and the currently, and most widely used, M8060 filter tape. For performing this analysis, we compared the attenuation measurements from AE33 with the absorption coefficients measured with different filter-based techniques. On-line co-located multi-angle absorption photometer (MAAP) measurements and off-line PP_UniMI polar photometer measurements were employed as reference absorption measurements for this work. To this aim, we used data from three different measurement stations located in the north-east of Spain, namely an urban background station (Barcelona, BCN), a regional background station (Montseny, MSY) and a mountaintop station (Montsec d'Ares, MSA). The median C values (at 637 nm) measured at the three stations ranged between 2.29 (at BCN and MSY, lowest 5th percentile of 1.97 and highest 95th percentile of 2.68) and 2.51 (at MSA, lowest 5th percentile of 2.06 and highest 95th percentile of 3.06). The analysis of the cross-sensitivity to scattering, for the two filter tapes considered here, revealed a large increase in the C factor when the single-scattering albedo (SSA) of the collected particles was above a given threshold, up to a 3-fold increase above the average C values. The SSA threshold appeared to be site dependent and ranged between 0.90 to 0.95 for the stations considered in the study. The results of the cross-sensitivity to scattering displayed a fitted constant multiple-scattering parameter, Cf, of 2.21 and 1.96, and a cross-sensitivity factor, ms, of 1.8 % and 3.4 % for the MSY and MSA stations, respectively, for the TFE-coated glass filter tape. For the M8060 filter tape, Cf values of 2.50, 1.96 and 1.82 and ms values of 1.6 %, 3.0 % and 4.9 % for the BCN, MSY and MSA stations, respectively, were obtained. SSA variations also influenced the spectral dependence of C, which showed an increase with wavelength when SSA was above the site-dependent threshold. Below the SSA threshold, no statistically significant dependence of C on the wavelength was observed. For the measurement stations considered here, the wavelength dependence of C was to some extent driven by the presence of dust particles during Saharan dust outbreaks that had the potential to increase the SSA above the average values. At the mountaintop station, an omission of the wavelength dependence of the C factor led to an underestimation of the absorption Ångström exponent (AAE) by up to 12 %. Differences in the absorption coefficient determined from AE33 measurements at BCN, MSY and MSA of around 35 %–40 % can be expected when using the site-dependent experimentally obtained C value instead of the nominal C value. Due to the fundamental role that the SSA of the particles collected on the filter tape has in the multiple-scattering parameter C, we present a methodology that allows the recognition of the conditions upon which the use of a constant and wavelength-independent C is feasible.
Ključne besede: black carbon, aerosol absorption, filter photometer, artifact
Objavljeno v RUNG: 01.10.2021; Ogledov: 2061; Prenosov: 0
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