1. Tunable emissive ▫$CsPbBr_3 /Cs_4PbBr_6$▫ quantum dots engineered by discrete phase transformation for enhanced photogating in field-effect phototransistorsHan Xiao, Siyuan Wan, Lin He, Junlong Zou, Andraž Mavrič, Yixi Wang, Marek Piotrowski, Anil Kumar Bandela, Paolo Samorì, Zhiming M. Wang, 2024, original scientific article Abstract: Precise control of quantum structures in hybrid nanocrystals requires advancements in scientific methodologies. Here, on the design of tunable CsPbBr3/Cs4PbBr6 quantum dots are reported by developing a unique discrete phase transformation approach in Cs4PbBr6 nanocrystals. Unlike conventional hybrid systems that emit solely in the green region, this current strategy produces adjustable luminescence in the blue (450 nm), cyan (480 nm), and green (510 nm) regions with high photoluminescence quantum yields up to 45%, 60%, and 85%, respectively. Concentration‐dependent studies reveal that phase transformation mechanisms and the factors that drive CsBr removal occur at lower dilutions while the dissolution–recrystallization process dominates at higher dilutions. When the polymer‐CsPbBr3/Cs4PbBr6 integrated into a field‐effected transistor the resulting phototransistors featured enhanced photosensitivity exceeding 105, being the highest reported for an n‐type phototransistor, while maintaining good transistor performances as compared to devices consisting of polymer‐CsPbBr3 NCs.
Keywords: crystallization mechanisms, dilution-induced kinetic trapping, photogating effect, phototransistors, quantum dots
Published in RUNG: 26.06.2024; Views: 674; Downloads: 9
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2. Multiresponsive nonvolatile memories based on optically switchable ferroelectric organic field-effect transistorsMarco Carroli, Alex Dixon, Martin Herder, Egon Pavlica, Stefan Hecht, Gvido Bratina, Emanuele Orgiu, Paolo Samorì, 2021, original scientific article Abstract: Organic transistors are key elements for flexible, wearable, and biocompatible logic applications. Multiresponsivity is highly sought‐after in organic electronics to enable sophisticated operations and functions. Such a challenge can be pursued by integrating more components in a single device, each one responding to a specific external stimulus. Here, the first multiresponsive organic device based on a photochromic–ferroelectric organic field‐effect transistor, which is capable of operating as nonvolatile memory with 11 bit memory storage capacity in a single device, is reported. The memory elements can be written and erased independently by means of light or an electric field, with accurate control over the readout signal, excellent repeatability, fast response, and high retention time. Such a proof of concept paves the way toward enhanced functional complexity in optoelectronics via the interfacing of multiple components in a single device, in a fully integrated low‐cost technology compatible with flexible substrates.
Keywords: organic transistors, memory, time-dependent
Published in RUNG: 11.03.2021; Views: 2840; Downloads: 0
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3. Fast-Response Photonic Device Based on Organic-Crystal Heterojunctions Assembled into a Vertical-Yet-Open Asymmetric ArchitectureLei Zhang, Egon Pavlica, Zhong, Xiaolan, Liscio Fabiola, LI Songlin, Gvido Bratina, Orgiu Emanuele, Samori Paolo, 2017, original scientific article Keywords: organski polprevodniki, merjenja časa preleta, organski fotodetektorji
Published in RUNG: 24.01.2017; Views: 4753; Downloads: 0
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4. Graphene-induced enhancement of n-type mobility in perylenediimide thin filmsGvido Bratina, Egon Pavlica, Srinivasa Rao Pathipati, Andrea Schlierf, Mirella El Gemayel, Paolo Samorì, Vincenzo PALERMO, 2014, original scientific article Keywords: grafen, transportne lastnosti, organski tankoslojni tranzistorji, tok fotovzbujenih nosilcev naboja
Published in RUNG: 16.06.2016; Views: 5388; Downloads: 135
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