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Role of transport band edge variation on delocalized charge transport in high-mobility crystalline organic semiconductors
Gvido Bratina, Andrey Kadashchuk, Egon Pavlica, Fei Tong, 2017, original scientific article

Abstract: We demonstrate that the degree of charge delocalization has a strong impact on polarization energy and thereby on the position of the transport band edge in organic semiconductors. This gives rise to long-range potential fluctuations, which govern the electronic transport through delocalized states in organic crystalline layers. This concept is employed to formulate an analytic model that explains a negative field dependence coupled with a positive temperature dependence of the charge mobility observed by a lateral time-of-flight technique in a high-mobility crystalline organic layer. This has important implications for the further understanding of the charge transport via delocalized states in organic semiconductors.
Keywords: organic semiconducotrs, time of flight, transport
Published in RUNG: 13.09.2017; Views: 4213; Downloads: 0
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