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1.
A systematically selected sample of luminous, long-duration, ambiguous nuclear transients
P. Wiseman, R. D. Williams, I. Arcavi, L. Galbany, M. J. Graham, S. Hönig, M. Newsome, B. Subrayan, Mark Sullivan, Tanja Petrushevska, 2025, izvirni znanstveni članek

Opis: ABSTRACT We present a search for luminous long-duration ambiguous nuclear transients (ANTs) similar to the unprecedented discovery of the extreme ambiguous event AT2021lwx with a $\gt 150$ d rise time and luminosity $10^{45.7}$ erg s$^{-1}$. We use the Lasair transient broker to search Zwicky Transient Facility (ZTF) data for transients lasting more than one year and exhibiting smooth declines. Our search returns 59 events, 7 of which we classify as ANTs assumed to be driven by accretion onto supermassive black holes. We propose the remaining 52 are stochastic variability from regular supermassive black hole accretion rather than distinct transients. We supplement the seven ANTs with three nuclear transients in ZTF that fail the light curve selection but have clear single flares and spectra that do not resemble typical active galactic nucleus. All of these 11 ANTs have a mid-infrared flare from an assumed dust echo, implying the ubiquity of dust around the black holes giving rise to ANTs. No events are more luminous than AT2021lwx, but one (ZTF19aamrjar) has twice the duration and a higher integrated energy release. On the other extreme, ZTF20abodaps reaches a luminosity close to AT2021lwx with a rise time $\lt 20$ d and that fades smoothly in $\gt 600$ d. We define a portion of rise-time versus flare amplitude space that selects ANTs with $\sim 50$ per cent purity against variable AGNs. We calculate a volumetric rate of $\gtrsim 3\times 10^{-11}$ Mpc$^{-1}$ yr$^{-1}$, consistent with the events being caused by tidal disruptions of intermediate and high-mass stars.
Ključne besede: tidal disruption events, accretion
Objavljeno v RUNG: 06.02.2025; Ogledov: 398; Prenosov: 8
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Comparing magnetism in isostructural oxides A[sub](0.8)La[sub](1.2)MnO[sub](4.1) : anisotropic spin glass (A = Ba) versus long range order (A = Sr)
Mirela Dragomir, Paul A. Dube, Iztok Arčon, Chad Boyer, Meghan Rutherford, Christopher Wiebe, Graham King, Hanna Dabkowska, John E. Greedan, 2019, izvirni znanstveni članek

Opis: This study presents the strikingly distinct magnetic properties of two isostructural compounds, Ba0.8La1.2MnO4.1 and Sr0.8La1.2MnO4.1 (K2NiF4 type, I4/mmm). Spectroscopic studies have shown that Mn is in a +3.0(1) oxidation state only, in both compounds; therefore, the charge is balanced by accommodating extra oxygen at interstitial sites, as confirmed by neutron powder diffraction. We found that the Ba compound exhibits an exceedingly rare anisotropic spin glass behavior, Tg = 26.4(4) K, with the moment freezing along the c-axis only while the in-plane spin components remain dynamic well below Tg. Experimental results including neutron diffraction, heat capacity, and magnetic (dc and ac) measurements performed on an oriented single crystal support this conclusion. This is a remarkable result, the only other known example of an anisotropic spin glass being Fe2TiO5. The spin glass state in Ba0.8La1.2MnO4.1 is argued to arise due to competing antiferromagnetic and ferromagnetic 180° Mn3+−O−Mn3+ superexchange interactions. In contrast, the Sr analogue shows 2D antiferromagnetic correlations and long-range antiferromagnetic order below 95(1) K with a remarkably reduced ordered moment of 1.449(49) μB/Mn3+ instead of the ∼4 μB expected for an S = 2 ion.
Ključne besede: antiferomagnetiki, Mn XANES, struktura
Objavljeno v RUNG: 23.10.2019; Ogledov: 4236; Prenosov: 0
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5.
A feasibility study of the use of reactive tracers to determine outdoor daytime OH radical concentrations within the urban environment
Iain R. White, Damien Martin, K Fredrik Petersson, Stephen J Henshaw, Graham Nickless, Guy C Lloyd-Jones, Kevin C Clemitshaw, Dudley E Shallcross, 2014, izvirni znanstveni članek

Opis: Using a specifically designed chemical tracer to indirectly measure local atmospheric hydroxyl radical (OH) concentrations is a very appealing concept. Such a tracer will provide information on the amount of OH a tracer encounters, as it moves through the urban environment and provide a stringent test of models. However, to date an outdoor experiment such as this has not been conducted. This article discusses the reasons why this is so and examines the feasibility of using tracers to measure integrated urban OH levels over short (≤1km) distances.
Ključne besede: reactive tracers, OH radicals, NO3 radicals, oxidising rate, dispersion, urban
Objavljeno v RUNG: 18.07.2019; Ogledov: 4178; Prenosov: 0
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Tracer concentration profiles measured in central London as part of the REPARTEE campaign
Damien Martin, K Fredrik Petersson, Iain R. White, Stephen H Henshaw, Graham Nickless, Amy Lovelock, Janet F Barlow, Tyrone Dunbar, Curtis R Wood, Dudley E. Shallcross, 2011, izvirni znanstveni članek

Opis: There have been relatively few tracer experiments carried out that have looked at vertical plume spread in urban areas. In this paper we present results from two tracer (cyclic perfluorocarbon) experiments carried out in 2006 and 2007 in central London centred on the BT Tower as part of the REPARTEE (Regent's Park and Tower Environmental Experiment) campaign. The height of the tower gives a unique opportunity to study vertical dispersion profiles and transport times in central London. Vertical gradients are contrasted with the relevant Pasquill stability classes. Estimation of lateral advection and vertical mixing times are made and compared with previous measurements. Data are then compared with a simple operational dispersion model and contrasted with data taken in central London as part of the DAPPLE campaign. This correlates dosage with non-dimensionalised distance from source. Such analyses illustrate the feasibility of the use of these empirical correlations over these prescribed distances in central London.
Ključne besede: advection, concentration (composition), dispersion, tracer, urban atmosphere, vertical mixing, vertical profile
Objavljeno v RUNG: 18.07.2019; Ogledov: 4453; Prenosov: 0
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7.
Use of reactive tracers to determine ambient OH radical concentrations: Application within the indoor environment
Iain R. White, Damien Martin, Maria Paz Muñoz, Fredrik K Petersson, Stephen J Henshaw, Graham Nickless, Guy C Lloyd-Jones, Keven C Clemitshaw, Dudley E. Shallcross, 2010, izvirni znanstveni članek

Opis: The hydroxyl radical (OH) plays a key role in determining indoor air quality. However, its highly reactive nature and low concentration indoors impede direct analysis. This paper describes the techniques used to indirectly quantify indoor OH, including the development of a new method based on the instantaneous release of chemical tracers into the air. This method was used to detect ambient OH in two indoor seminar rooms following tracer detection by gas chromatography- mass spectrometry (GCMS). The results from these tests add to the small number of experiments that have measured indoor OH which are discussed with regard to future directions within air quality research.
Ključne besede: Ozone, Indoor air pollution, Indoor ozone, chemical tracers
Objavljeno v RUNG: 18.07.2019; Ogledov: 4182; Prenosov: 0
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8.
Urban tracer dispersion experiments during the second DAPPLE field campaign in London 2004
Damien Martin, Catheryn S Price, Iain R. White, Graham Nickless, K Fredrik Petersson, Rex E Britter, Alan G Robins, Stephen E Belcher, Janet F Barlow, Marie Neophytou, Samantha J Arnold, Alan S Tomlin, Robert J Smalley, Dudley E. Shallcross, 2010, izvirni znanstveni članek

Opis: As part of the DAPPLE programme two large scale urban tracer experiments using multiple simultaneous releases of cyclic perfluoroalkanes from fixed location point sources was performed. The receptor concentrations along with relevant meteorological parameters measured are compared with a three screening dispersion models in order to best predict the decay of pollution sources with respect to distance. It is shown here that the simple dispersion models tested here can provide a reasonable upper bound estimate of the maximum concentrations measured with an empirical model derived from field observations and wind tunnel studies providing the best estimate. An indoor receptor was also used to assess indoor concentrations and their pertinence to commonly used evacuation procedures.
Ključne besede: Dapple, dispersion
Objavljeno v RUNG: 18.07.2019; Ogledov: 3983; Prenosov: 0
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9.
CityFlux perfluorocarbon tracer experiments
Fredrik K Petersson, Damien Martin, Iain R. White, Stephen J Henshaw, Graham Nickless, Ian Longley, Carl J Percival, Martin Gallagher, Dudley E. Shallcross, 2010, izvirni znanstveni članek

Opis: In June 2006, two perfluorocarbon tracer experiments were conducted in central Manchester UK as part of the CityFlux campaign. The main aim was to investigate vertical dispersion in an urban area during convective conditions, but dispersion mechanisms within the street network were also studied. Paired receptors were used in most cases where one receptor was located at ground level and one at roof level. One receptor was located on the roof of Portland Tower which is an 80m high building in central Manchester. Source receptor distances in the two experiments varied between 120 and 600 m. The results reveal that maximum concentration was sometimes found at roof level rather than at ground level implying the effectiveness of convective forces on dispersion. The degree of vertical dispersion was found to be dependent on source receptor distance as well as on building height in proximity to the release site. Evidence of flow channelling in a street canyon was also found. Both a Gaussian profile and a street network model were applied and the results show that the urban topography may lead to highly effective flow channelling which therefore may be a very important dispersion mechanism should the right meteorological conditions prevail. The experimental results from this campaign have also been compared with a simple urban dispersion model that was developed during the DAPPLE framework and show good agreement with this. The results presented here are some of the first published regarding vertical dispersion. More tracer experiments are needed in order to further characterise vertical concentration profiles and their dependence on, for instance, atmospheric stability. The impact of urban topography on pollutant dispersion is important to focus on in future tracer experiments in order to improve performance of models as well as for our understanding of the relationship between air quality and public health.
Ključne besede: air quality, atmospheric chemistry, concentration (composition), convective system, dispersion, public health, street canyon, tracer, urban area
Objavljeno v RUNG: 18.07.2019; Ogledov: 4169; Prenosov: 0
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10.
Year-long measurements of C1-C3 halocarbons at an urban site and their relationship with meteorological parameters
M Anwar K Khan, M Iqbal Mead, Iain R. White, Ben Golledge, Graham Nickless, Alan Knights, Damien Martin, Alison C Rivett, Brian G R Greally, Dudley E Shallcross, 2009, izvirni znanstveni članek

Opis: The mixing ratios of 11 C1–C3 halocarbons have been measured using a GC–twin‐linked ECD system over the period from October 2004 to December 2005 at an urban site in Bristol, UK. Time series and seasonal variations of the halocarbons were analysed over the period to determine biogenic and anthropogenic sources and sinks. Correlations between the target halocarbons were also observed, suggesting common sources within the area. Wind rose plots for all halocarbons have been used to assist in the determination of halocarbons sources. Halocarbon concentrations are highest at low‐wind speeds and decrease as wind speed increases, a few species (CCl4 and CH3Cl most notably) rise at very high‐wind speeds suggesting release from the Bristol Channel.
Ključne besede: adsorption–desorption system, anthropogenic halocarbons, biogenic halocarbons, electron capture detector, gas chromatography, methyl bromide
Objavljeno v RUNG: 18.07.2019; Ogledov: 4075; Prenosov: 0
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