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1.
Hydrazone-linked covalent organic framework catalyst via efficient Pd recovery from wastewater
Mahira Bashri, Sushil Kumar, Pallab Bhandari, Sasi Stephen, Matthew J. O'Connor, Safa Gaber, Tina Škorjanc, Matjaž Finšgar, Gisha Elizabeth Luckachan, Blaž Belec, 2024, izvirni znanstveni članek

Opis: Global consumption and discharge of palladium (Pd) have raised environmental concerns but also present an opportunity for the sustainable recovery and reuse of this precious metal. Adsorption has proven to be an efficient method for the selective recovery of Pd from industrial wastewater. This study investigated a hydrazone-linked covalent organic framework (Tfpa-Od COF) as a potential material for the high-affinity adsorption of Pd2+ ions from wastewater, achieving a Kd value of 3.62 × 106 mL g–1. The electron-rich backbone of the COF contributes to its excellent selective removal efficiency (up to 100%) and adsorption capacity of 372.59 mg g–1. Furthermore, the Pd-adsorbed COF was evaluated as a sustainable catalyst for the Suzuki–Miyaura coupling reaction, demonstrating good catalytic conversion and recyclability. This work attempts to showcase a protocol for reusing waste palladium generated in water to fabricate heterogeneous catalysts and, thereby, promote the circular economy concept.
Ključne besede: covalent organic frameworks, sustainability, catalysis, palladium adsorption, water purification
Objavljeno v RUNG: 22.08.2024; Ogledov: 746; Prenosov: 6
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2.
Tunable emissive ▫$CsPbBr_3 /Cs_4PbBr_6$▫ quantum dots engineered by discrete phase transformation for enhanced photogating in field-effect phototransistors
Han Xiao, Siyuan Wan, Lin He, Junlong Zou, Andraž Mavrič, Yixi Wang, Marek Piotrowski, Anil Kumar Bandela, Paolo Samorì, Zhiming M. Wang, 2024, izvirni znanstveni članek

Opis: Precise control of quantum structures in hybrid nanocrystals requires advancements in scientific methodologies. Here, on the design of tunable CsPbBr3/Cs4PbBr6 quantum dots are reported by developing a unique discrete phase transformation approach in Cs4PbBr6 nanocrystals. Unlike conventional hybrid systems that emit solely in the green region, this current strategy produces adjustable luminescence in the blue (450 nm), cyan (480 nm), and green (510 nm) regions with high photoluminescence quantum yields up to 45%, 60%, and 85%, respectively. Concentration‐dependent studies reveal that phase transformation mechanisms and the factors that drive CsBr removal occur at lower dilutions while the dissolution–recrystallization process dominates at higher dilutions. When the polymer‐CsPbBr3/Cs4PbBr6 integrated into a field‐effected transistor the resulting phototransistors featured enhanced photosensitivity exceeding 105, being the highest reported for an n‐type phototransistor, while maintaining good transistor performances as compared to devices consisting of polymer‐CsPbBr3 NCs.
Ključne besede: crystallization mechanisms, dilution-induced kinetic trapping, photogating effect, phototransistors, quantum dots
Objavljeno v RUNG: 26.06.2024; Ogledov: 922; Prenosov: 11
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3.
Complex network based Fourier analysis for signal processing
Vijayan Vijesh, K. Satheesh Kumar, Mohanachandran Nair Sindhu Swapna, Sankaranarayana Iyer Sankararaman, 2024, objavljeni znanstveni prispevek na konferenci

Ključne besede: fourier analysis, complex network, signal processing
Objavljeno v RUNG: 15.04.2024; Ogledov: 1409; Prenosov: 3
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4.
Markov chain approach to rectifier circuits
Vijayan Vijesh, K. Satheesh Kumar, Mohanachandran Nair Sindhu Swapna, Sankaranarayana Iyer Sankararaman, 2024, objavljeni znanstveni prispevek na konferenci

Ključne besede: Markov chain, rectifier, graph theory
Objavljeno v RUNG: 15.04.2024; Ogledov: 1444; Prenosov: 3
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5.
Wavelength-resolved reverberation mapping of quasar CTS C30.10: Dissecting Mg II and Fe II emission regions
Raj Prince, Michal Zajaček, Bożena Czerny, Piotr Trzcionkowski, Mateusz Bronikowski, Catalina Sobrino Figaredo, Swayamtrupta Panda, Mary Loli Martinez-Aldama, Krzysztof Hryniewicz, Vikram Kumar Jaiswal, Marzena Śniegowska, Mohammad-Hassan Naddaf, Maciej Bilicki, Martin Haas, Marek Jacek Sarna, Vladimir Karas, Aleksandra Olejak, Robert Przyłuski, Mateusz Rałowski, Andrzej Udalski, Ramotholo R. Sefako, Anja Genade, Hannah L. Worters, 2022, izvirni znanstveni članek

Opis: Context. We present the results of the reverberation monitoring of the Mg II broad line and Fe II pseudocontinuum for the luminous quasar CTS C30.10 (z = 0.90052) with the Southern African Large Telescope in 2012–2021. Aims. We aimed at disentangling the Mg II and UV Fe II variability and the first measurement of UV Fe II time delay for a distant quasar. Methods. We used several methods for the time-delay measurements and determined the Fe II and Mg II time delays. We also performed a wavelength-resolved time delay study for a combination of Mg II and Fe II in the 2700–2900 Å rest-frame wavelength range. Results. We obtain a time delay for Mg II of 275.5−19.5+12.4 days in the rest frame, and we have two possible solutions of 270.0−25.3+13.8 days and 180.3−30.0+26.6 in the rest frame for Fe II. Combining this result with the old measurement of Fe II UV time delay for NGC 5548, we discuss for first time the radius-luminosity relation for UV Fe II with the slope consistent with 0.5 within the uncertainties. Conclusions. Because the Fe II time delay has a shorter time-delay component but the lines are narrower than Mg II, we propose that the line-delay measurement is biased toward the part of the broad line region (BLR) facing the observer. The bulk of the Fe II emission may arise from the more distant BLR region, however, the region that is shielded from the observer.
Ključne besede: accretion, accretion disks / quasars: emission lines / quasars: individual: CTS C30.10 / techniques: spectroscopic / techniques: photometric
Objavljeno v RUNG: 13.11.2023; Ogledov: 1783; Prenosov: 5
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6.
Wavelength-resolved reverberation mapping of intermediate-redshift quasars HE 0413-4031 and HE 0435-4312 : dissecting Mg II, optical Fe II, and UV Fe II emission regions
Raj Prince, Michal Zajaček, Swayamtrupta Panda, Krzysztof Hryniewicz, Vikram Kumar Jaiswal, Bożena Czerny, Piotr Trzcionkowski, Mateusz Bronikowski, Mateusz Rałowski, Catalina Sobrino Figaredo, 2023, izvirni znanstveni članek

Opis: Context. We present the wavelength-resolved reverberation mapping (RM) of combined Mg II and UV Fe II broad-line emissions for two intermediate-redshift (z ∼ 1), luminous quasars, HE 0413-4031 and HE 0435-4312, monitored by the Southern African Large Telescope (SALT) and 1m class telescopes between 2012 and 2022. Aims. Using a wavelength-resolved technique, we aim to disentangle the Mg II and Fe II emission regions and to build a radius–luminosity (R–L) relation for UV Fe II emission, which has so far remained unconstrained. Methods. We applied several time-delay methodologies to constrain the time delays for total Mg II and Fe II emissions. In addition, wavelength-resolved RM is performed to quantify the inflow or outflow of broad-line region (BLR) gas around the supermassive black hole and to disentangle the emission and the emitting regions based on lines produced in proximity to each other. Results. The mean total FeII time delay is nearly equal to the mean total MgII time delay for HE 0435-4312, suggesting the co-spatiality of their emission regions. However, in HE 0413-4031, the mean FeII time delay is found to be longer than the mean MgII time delay, suggesting that FeII emission is produced at greater distances from the black hole. The UV FeII R–L relation is updated with these two quasars (now four in total) and compared with the optical FeII relation (20 sources), which suggests that the optical FeII emission region is located further than the UV FeII region by a factor of 1.7–1.9, that is, RFeII-opt ∼ (1.7 − 1.9)RFeII-UV. Conclusion. Wavelength-resolved reverberation is an efficient way to constrain the geometry and structure of the BLR. We detected a weak pattern in the time delay versus wavelength relation, suggesting that the MgII broad line originates from a region slightly closer to the SMBH than the UV FeII pseudo continuum, although the difference is not very significant. Comparison of MgII, UV, and optical FeII R–L relations suggests that the difference may be greater for lower-luminosity sources, possibly with the MgII emission originating further from the SMBH. In the future, more RM data will be acquired, allowing better constraints on these trends, in particular the UV FeII R–L relation.
Ključne besede: accretion, accretion disks, emission lines, photometric, spectroscopic
Objavljeno v RUNG: 13.11.2023; Ogledov: 1946; Prenosov: 5
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7.
8.
Modulation of charge transfer exciton dynamics in organic semiconductors using different structural arrangements
Cristian Soncini, Abhishek Kumar, Federica Bondino, Elena Magnano, Matija Stupar, Barbara Ressel, Giovanni De Ninno, Antonis Papadopoulos, Efthymis Serpetzoglou, Emmanuel Stratakis, Maddalena Pedio, 2023, izvirni znanstveni članek

Opis: In devices based on organic semiconductors, aggregation and inter-molecular interactions play a key role in affecting the photo-physical and dynamical carrier properties of the material, potentially becoming a limiting factor to achieving high efficiency. As a consequence, a detailed understanding of the interplay between the film molecular structure and the material properties is essential to properly design devices with optimized performance. Here we demonstrate how different molecular structural arrangements modulate the charge transfer (CT) dynamics in cobalt phthalocyanine (CoPc) thin films. By transient absorption spectroscopy and time-resolved photoemission spectroscopy, we study the influence of different CoPc structures on the dynamical electronic properties, the CoPc intra and inter- molecular de-excitation pathways up to 7 ns. We rationalize the ultrafast formation of triplet states in the CoPc through an electron exchange process between the single-occupied Co3dz2 orbital and p orbitals of the macrocycle, which obviate for an energetically unfavourable spin-flip. We found enhanced CT exciton lifetime in the case of the herringbone structure with respect to the brickwork one, possibly explainable by a more efficient CT exciton delocalization along the stacking axis.
Ključne besede: charge transfer, organic molecules, time resolved spectroscopies
Objavljeno v RUNG: 30.06.2023; Ogledov: 2212; Prenosov: 8
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9.
10.
Markov chain approach to rectifier circuits
Mohanachandran Nair Sindhu Swapna, Vijayan Vijesh, K. Satheesh Kumar, Sankaranarayana Iyer Sankararaman, 2022, objavljeni povzetek znanstvenega prispevka na konferenci

Ključne besede: Markov chain, rectifier circuits, graph theory
Objavljeno v RUNG: 19.12.2022; Ogledov: 1702; Prenosov: 0
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