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Opis: The aim of the dissertation was to study aerosol loading distributions and properties over the Vipava valley, a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin. An infrared Mie and a two-wavelength polarization Raman lidar systems were used as main detection tools. The polarization Raman lidar, which provides the capability to extract the extinction coefficient, backscatter coefficients, depolarization ratio, backscatter Ångström exponent, lidar ratio and water vapor mixing ratio profiles, was itself designed, built and calibrated as a part of this thesis. Lidar data, combined with in-situ measurements, was used to determine detailed information on different aerosol types. Vertical profiles of aerosol mass concentration were extracted from the Mie lidar data taken in April 2016, where the in-situ measurements of aerosol size distribution and number concentration as well as aerosol absorption coefficient and black carbon mass concentration were used to estimate the mass extinction efficiency (MEE). Aerosol morphology and chemical composition determined by SEM-EDX on sampled particles were used for the identification of primary aerosol types. Two cases with different atmospheric conditions (long range mineral dust transport and local biomass burning) and different expected the dominant presence of specific aerosol types (mineral dust and soot) were investigated in more detail. They revealed significantly different aerosol properties and distributions within the valley, affecting radiative heat exchange. A more detailed investigation of aerosol properties throughout the troposphere in different atmospheric conditions was made possible by the two-wavelength polarization Raman lidar system, deployed in Ajdovščina (town of Vipava valley) from September 2017. Using its aerosol identification capabilities, based on particle depolarization ratio and lidar ratio measurements, it was possible to identify predominant aerosol types in the observed atmospheric structures, for example in different atmospheric layers in the case of the stratified atmosphere. Primary anthropogenic aerosols within the valley were found to be mainly emitted from two sources: individual domestic heating systems, which mostly use biomass fuel and traffic. Natural aerosols, transported over large distances, such as mineral dust and sea salt, were observed both above and entering into the planetary boundary layer. Backscatter contribution of each aerosol type was separated and the corresponding extinction contribution was derived from lidar observations.
Ključne besede: Vipava valley, aerosol distribution, aerosol characterization, lidar remote sensing, in-situ measurements, aerosol loading.
Objavljeno v RUNG: 23.10.2018; Ogledov: 7398; Prenosov: 157
Celotno besedilo (29,39 MB)

Opis: Presence of atmospheric aerosols affects the Earth’s radiation budget and thus also atmospheric thermal structure, which in turn affects cloud and planetary boundary layer (PBL) dynamics. We combine in-situ and remote measurements to determine aerosol properties in a representative hot-spot for air pollution in a complex terrain configuration. Vertical profiles of aerosol properties were investigated using a two-wavelength polarization Raman lidar system in the Vipava valley. Using lidar-obtained particle depolarization ratio, lidar ratio and backscatter Ångström exponent (355 nm / 1064 nm), which depend on aerosol shape, size and refractive index, thus the aerosols can be identified and the roles of different aerosol types in the observed atmospheric processes were investigated. In addition, aerosol absorption coefficients were measured in-situ by Aethalometers (AE33, Magee Scientific / Aerosol d.o.o.) on the valley floor and on the adjacent mountain range, 850 m above the lidar site. Our primary goal was to study the variability of aerosol types within and above the Vipava valley, which was performed using the entire lidar dataset from August – December 2017. Primary anthropogenic aerosols within the valley is mainly emitted from two sources: individual domestic heating systems, which mostly use biomass fuel and traffic. Natural aerosols, transported by long-range transport, such as mineral dust and sea salt, were observed both above the PBL and entering into the PBL. Vertical distributions of aerosol properties, in par- ticular the particle depolarization ratio, indicated atmospheric stratification with different aerosol types occupying different height ranges. In the presence of Bora (strong down-slope wind), Kelvin-Helmholtz instabilities were observed between the PBL and the free troposphere. Using aerosol type identification capability of our system, we discovered that this instability was responsible for ejecting aerosols from the PBL up to 2 km into the free troposphere. In addition, we improved the reliability of aerosol identification in vertical profiles using absorption coeffi- cient measured by Aethalometer. Combining it with the aerosol extinction coefficient at 355 nm derived from lidar data, we derived aerosol single scattering albedo (SSA), which is an important parameter for aerosol characterization.
Ključne besede: Aerosol, Vipava valley, lidar
Objavljeno v RUNG: 23.04.2018; Ogledov: 4383; Prenosov: 0
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Objavljeno v RUNG: 21.07.2017; Ogledov: 5037; Prenosov: 0
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Ključne besede: ZnO Nanorod Arrays, ITO-PET, solution growth
Objavljeno v RUNG: 16.01.2017; Ogledov: 4697; Prenosov: 0
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Opis: The Vipava valley in Slovenia is well known for the appearance of strong, gusty North-East Bora winds, which occur as a result of air flows over an adjacent orographic barrier. There are three revealing wind directions within the valley which were found to give rise to specific types of atmospheric structures. These structures were investigated using a Mie scattering lidar operating at 1064 nm, which provided high temporal and spatial resolution backscatter data on aerosols, which were used as tracers for atmospheric flows. Wind properties were monitored at the bottom of the valley and at the rim of the barrier using two ultrasonic anemometers. Twelve time periods between February and April 2015 were selected when lidar data was available. The periods were classified according to the wind speed and direction and investigated in terms of appearance of atmospheric structures. In two periods with strong or moderate Bora, periodic atmospheric structures in the lidar data were observed at heights above the mountain barrier and are believed to be Kelvin–Helmholtz waves, induced by wind shear. No temporal correlation was found between these structures and wind gusts at the ground level. The influence of the wind on the height of the planetary boundary layer was studied as well. In periods with low wind speeds, the vertical evolution of the planetary boundary layer was found to be governed by solar radiation and clouds. In periods with strong or moderate Bora wind, convection within the planetary boundary layer was found to be much weaker due to strong turbulence close to the ground, which inhibited mixing through the entire layer.
Ključne besede: Downslope wind Lidar observations Kelvin–Helmholtz waves Bora
Objavljeno v RUNG: 06.01.2017; Ogledov: 5399; Prenosov: 0
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