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51.
Distribution of gaseous and particulate organic composition during dark α-pinene ozonolysis
Marie Camredon, Jacqueline F Hamilton, Mohammed S Alam, Kevin P Wyche, Timo Carr, Iain R. White, Paul S Monks, Andrew R Rickard, William J Bloss, 2010, izvirni znanstveni članek

Opis: Secondary Organic Aerosol (SOA) affects atmospheric composition, air quality and radiative transfer, however major difficulties are encountered in the development of reliable models for SOA formation. Constraints on processes involved in SOA formation can be obtained by interpreting the speciation and evolution of organics in the gaseous and condensed phase simultaneously. In this study we investigate SOA formation from dark α-pinene ozonolysis with particular emphasis upon the mass distribution of gaseous and particulate organic species. A detailed model for SOA formation is compared with the results from experiments performed in the EUropean PHOtoREactor (EUPHORE) simulation chamber, including on-line gas-phase composition obtained from Chemical-Ionization-Reaction Time-Of-Flight Mass-Spectrometry measurements, and off-line analysis of SOA samples performed by Ion Trap Mass Spectrometry and Liquid Chromatography. The temporal profile of SOA mass concentration is relatively well reproduced by the model. Sensitivity analysis highlights the importance of the choice of vapour pressure estimation method, and the potential influence of condensed phase chemistry. Comparisons of the simulated gaseous-and condensed-phase mass distributions with those observed show a generally good agreement. The simulated speciation has been used to (i) propose a chemical structure for the principal gaseous semi-volatile organic compounds and condensed monomer organic species, (ii) provide evidence for the occurrence of recently suggested radical isomerisation channels not included in the basic model, and (iii) explore the possible contribution of a range of accretion reactions occurring in the condensed phase. We find that oligomer formation through esterification reactions gives the best agreement between the observed and simulated mass spectra
Ključne besede: Aerosol, Aerosol formation, Smog chamber
Objavljeno v RUNG: 18.07.2019; Ogledov: 2842; Prenosov: 0
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52.
53.
Investigation of Aerosol Properties and Structures in Two Representative Meteorological Situations over the Vipava Valley Using Polarization Raman LiDAR
Longlong Wang, Samo Stanič, William Eichinger, Griša Močnik, Luka Drinovec, Asta Gregorič, 2019, izvirni znanstveni članek

Opis: Vipava valley in Slovenia is a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin. Aerosol loading distributions and optical properties were investigated using a two-wavelength polarization Raman LiDAR, which provided extinction coefficient, backscatter coefficient, depolarization ratio, backscatter Ångström exponent and LiDAR ratio profiles. Two different representative meteorological situations were investigated to explore the possibility of identifying aerosol types present in the valley. In the first case, we investigated the effect of strong downslope (Bora) wind on aerosol structures and characteristics. In addition to observing Kelvin–Helmholtz instability above the valley, at the height of the adjacent mountain ridge, we found new evidence for Bora-induced processes which inject soil dust aerosols into the free troposphere up to twice the height of the planetary boundary layer (PBL). In the second case, we investigated aerosol properties and distributions in stable weather conditions. From the observed stratified vertical aerosol structure and specific optical properties of different layers we identified predominant aerosol types in these layers.
Ključne besede: aerosol structures, aerosol characterization, polarization Raman LiDAR, Vipava valley
Objavljeno v RUNG: 08.03.2019; Ogledov: 3812; Prenosov: 118
.pdf Celotno besedilo (3,11 MB)

54.
Properties of tropospheric aerosols observed over southwest Slovenia
Tingyao He, Yingying Chen, Samo Stanič, Klemen Bergant, Fei Gao, Dengxin Hua, 2018, izvirni znanstveni članek

Opis: From August to October 2010 lidar measurements of aerosols in the troposphere were performed at Otlica observatory, Slovenia, using a vertical scanning elastic lidar. The lidar data sample, which contains 38 nighttime vertical profiles of the mean aerosol extinction, was combined with continuous ozone concen- tration (O3), particulate matter concentrations (PM) and daily radiosonde data. The obtained radiosonde- and lidar-derived heights of the atmospheric boundary layer (ABL), which varied considerably from day to day, were found to be in good agreement. The mean values of the aerosol optical depth (AOD) at 355 nm, were calculated separately for the ABL and for the free troposphere (FT). A ten-fold increase of the FT AOD was observed during the days with predicted presence of Saharan dust above the lidar site. To correlate AOD values with the type and origin of aerosols, backward trajectories of air-masses above Otlica were modeled using the HYSPLIT model and clustered. High ABL AOD values were found to be correlated with local circulations and slowly approaching air masses from the Balkans and low values with northwestern flows. The highest values correlated with southwestern flows originating in northern Africa.
Ključne besede: Aerosol, Optical depth, Lidar, Atmospheric boundary layer
Objavljeno v RUNG: 22.02.2019; Ogledov: 3744; Prenosov: 0
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55.
Retrieval of Vertical Mass Concentration Distributions—Vipava Valley Case Study
Longlong Wang, Samo Stanič, Klemen Bergant, William Eichinger, Griša Močnik, Luka Drinovec, Janja Vaupotič, Miloš Miler, Mateja Gosar, Asta Gregorič, 2019, izvirni znanstveni članek

Opis: Aerosol vertical profiles are valuable inputs for the evaluation of aerosol transport models, in order to improve the understanding of aerosol pollution ventilation processes which drive the dispersion of pollutants in mountainous regions. With the aim of providing high-accuracy vertical distributions of particle mass concentration for the study of aerosol dispersion in small-scale valleys, vertical profiles of aerosol mass concentration for aerosols from different sources (including Saharan dust and local biomass burning events) were investigated over the Vipava valley, Slovenia, a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin. The analysis was based on datasets taken between 1–30 April 2016. In-situ measurements of aerosol size, absorption, and mass concentration were combined with lidar remote sensing, where vertical profiles of aerosol concentration were retrieved. Aerosol samples were characterized by SEM-EDX, to obtain aerosol morphology and chemical composition. Two cases with expected dominant presence of different specific aerosol types (mineral dust and biomass-burning aerosols) show significantly different aerosol properties and distributions within the valley. In the mineral dust case, we observed a decrease of the elevated aerosol layer height and subsequent spreading of mineral dust within the valley, while in the biomass-burning case we observed the lifting of aerosols above the planetary boundary layer (PBL). All uncertainties of size and assumed optical properties, combined, amount to the total uncertainty of aerosol mass concentrations below 30% within the valley. We have also identified the most indicative in-situ parameters for identification of aerosol type.
Ključne besede: valley air pollution, aerosol vertical distributions, lidar remote sensing, in-situ measurements, aerosol identification
Objavljeno v RUNG: 09.01.2019; Ogledov: 4110; Prenosov: 113
.pdf Celotno besedilo (7,43 MB)

56.
Aerosol monitoring over Vipava valley using Raman polarization lidar
Longlong Wang, Samo Stanič, Klemen Bergant, William Eichinger, Asta Gregorič, Griša Močnik, Luka Drinovec, 2018, objavljeni povzetek znanstvenega prispevka na konferenci

Opis: Vipava valley in southwest Slovenia is a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin in mountainous terrain. An investigation of aerosol properties throughout the troposphere in different atmospheric conditions was made possible by a deployment of a two-wavelength polarization Raman lidar system combining with in-situ measurements in the valley (in the town of Ajdovščina) from September 2017. Using its aerosol identification capabilities, which are based on particle depolarization ratio and lidar ratio measurements, it was possible to identify predominant aerosol types in the observed atmospheric structures, for example in different atmospheric layers in the case of stratified atmosphere. Primary anthropogenic aerosols within the valley were found to be mainly emitted from two sources: individual domestic heating systems, which mostly use biomass fuel, and from traffic. A considerable fraction of natural aerosols (for example mineral dust and sea salt), transported over large distances, were observed both above and entering into the planetary boundary layer. According to the properties of different aerosol types, backscatter contribution of each aerosol type was evaluated and the corresponding extinction contribution was derived from lidar observations. Statistical analysis of the presence of different aerosol types was performed on the entire available dataset from 2017 and 2018.
Ključne besede: lidar, aerosol type, Vipava valley
Objavljeno v RUNG: 03.12.2018; Ogledov: 4215; Prenosov: 0
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57.
STUDY OF ATMOSPHERIC AEROSOL PROPERTIES IN THE VIPAVA VALLEY
Longlong Wang, doktorska disertacija

Opis: The aim of the dissertation was to study aerosol loading distributions and properties over the Vipava valley, a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin. An infrared Mie and a two-wavelength polarization Raman lidar systems were used as main detection tools. The polarization Raman lidar, which provides the capability to extract the extinction coefficient, backscatter coefficients, depolarization ratio, backscatter Ångström exponent, lidar ratio and water vapor mixing ratio profiles, was itself designed, built and calibrated as a part of this thesis. Lidar data, combined with in-situ measurements, was used to determine detailed information on different aerosol types. Vertical profiles of aerosol mass concentration were extracted from the Mie lidar data taken in April 2016, where the in-situ measurements of aerosol size distribution and number concentration as well as aerosol absorption coefficient and black carbon mass concentration were used to estimate the mass extinction efficiency (MEE). Aerosol morphology and chemical composition determined by SEM-EDX on sampled particles were used for the identification of primary aerosol types. Two cases with different atmospheric conditions (long range mineral dust transport and local biomass burning) and different expected the dominant presence of specific aerosol types (mineral dust and soot) were investigated in more detail. They revealed significantly different aerosol properties and distributions within the valley, affecting radiative heat exchange. A more detailed investigation of aerosol properties throughout the troposphere in different atmospheric conditions was made possible by the two-wavelength polarization Raman lidar system, deployed in Ajdovščina (town of Vipava valley) from September 2017. Using its aerosol identification capabilities, based on particle depolarization ratio and lidar ratio measurements, it was possible to identify predominant aerosol types in the observed atmospheric structures, for example in different atmospheric layers in the case of the stratified atmosphere. Primary anthropogenic aerosols within the valley were found to be mainly emitted from two sources: individual domestic heating systems, which mostly use biomass fuel and traffic. Natural aerosols, transported over large distances, such as mineral dust and sea salt, were observed both above and entering into the planetary boundary layer. Backscatter contribution of each aerosol type was separated and the corresponding extinction contribution was derived from lidar observations.
Ključne besede: Vipava valley, aerosol distribution, aerosol characterization, lidar remote sensing, in-situ measurements, aerosol loading.
Objavljeno v RUNG: 23.10.2018; Ogledov: 7229; Prenosov: 157
.pdf Celotno besedilo (29,39 MB)

58.
Vertical profiling of aerosol properties with two-wavelength polarization Raman lidar over the Vipava valley
Longlong Wang, Samo Stamoč, Asta Gregorič, Griša Močnik, Luka Drinovec, Klemen Bergant, William Eichinger, 2018, objavljeni povzetek znanstvenega prispevka na konferenci

Opis: Presence of atmospheric aerosols affects the Earth’s radiation budget and thus also atmospheric thermal structure, which in turn affects cloud and planetary boundary layer (PBL) dynamics. We combine in-situ and remote measurements to determine aerosol properties in a representative hot-spot for air pollution in a complex terrain configuration. Vertical profiles of aerosol properties were investigated using a two-wavelength polarization Raman lidar system in the Vipava valley. Using lidar-obtained particle depolarization ratio, lidar ratio and backscatter Ångström exponent (355 nm / 1064 nm), which depend on aerosol shape, size and refractive index, thus the aerosols can be identified and the roles of different aerosol types in the observed atmospheric processes were investigated. In addition, aerosol absorption coefficients were measured in-situ by Aethalometers (AE33, Magee Scientific / Aerosol d.o.o.) on the valley floor and on the adjacent mountain range, 850 m above the lidar site. Our primary goal was to study the variability of aerosol types within and above the Vipava valley, which was performed using the entire lidar dataset from August – December 2017. Primary anthropogenic aerosols within the valley is mainly emitted from two sources: individual domestic heating systems, which mostly use biomass fuel and traffic. Natural aerosols, transported by long-range transport, such as mineral dust and sea salt, were observed both above the PBL and entering into the PBL. Vertical distributions of aerosol properties, in par- ticular the particle depolarization ratio, indicated atmospheric stratification with different aerosol types occupying different height ranges. In the presence of Bora (strong down-slope wind), Kelvin-Helmholtz instabilities were observed between the PBL and the free troposphere. Using aerosol type identification capability of our system, we discovered that this instability was responsible for ejecting aerosols from the PBL up to 2 km into the free troposphere. In addition, we improved the reliability of aerosol identification in vertical profiles using absorption coeffi- cient measured by Aethalometer. Combining it with the aerosol extinction coefficient at 355 nm derived from lidar data, we derived aerosol single scattering albedo (SSA), which is an important parameter for aerosol characterization.
Ključne besede: Aerosol, Vipava valley, lidar
Objavljeno v RUNG: 23.04.2018; Ogledov: 4255; Prenosov: 0
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59.
Procjena genotoksičnog potencijala uzoraka aerosola iz Tuzle
Maida Šljivić Husejnović, Dalila Imamović, Ermina Cilović, Aida Smajlović, Nahida Srabović, Martina Bergant Marušič, 2018, objavljeni znanstveni prispevek na konferenci

Ključne besede: aerozagađenje, genotoksičnost, zdravlje ljudi, aerosol, Tuzla
Objavljeno v RUNG: 30.03.2018; Ogledov: 3741; Prenosov: 0
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60.
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