11. Highly time-resolved apportionment of carbonaceous aerosols from wildfire using the TC-BC method : camp fire 2018 case studyMatic Ivančič, Martin Rigler, Bálint Alföldy, Gašper Lavrič, Irena Ježek, Asta Gregorič, 2023, izvirni znanstveni članek Ključne besede: black carbon, brown carbon, carbonaceous aerosol, wildfire, air quality, CASS
Objavljeno v RUNG: 06.06.2023; Ogledov: 1079; Prenosov: 10
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12. A METHOD FOR QUANTIFICATION OF MINERAL DUST IN AIR BASED ON OPTICAL ABSORPTION OF PARTICLES CONCENTRATED BY A VIRTUAL IMPACTOR AND A DEVICE PERFORMING THE SAID METHODLuka Drinovec, Griša Močnik, IASONAS STAVROULAS, SPIROS BEZANTAKOS, Michael Pikridas, FLORIN UNGA, JEAN SCIARE, patent Opis: The present invention belongs to the field of devices and methods for measurement of particle concentration, more precisely to the field of devices and methods for quantification of particles based ontheir physical characteristics, especially with the use of optical means. The invention relates to a method for determination of ambient mineral dust concentration based on optical absorption of particles concentrated by a virtual impactor as well as a device performing the said method. The method comprises the following steps: sampling air samples with particle size smaller than 1 mum (PM1) andsampling air samples with particle size up to 10 mum; concentrating the samples with particle sizes up to 10 mum with a virtual impactor; measuring optical absorption of collected samples at least onewavelength from UV to IR spectre, preferably from 370 to 950 nm, most preferably at 370 nm; subtracting the absorption of the samples with particle size smaller than 1 mum from the absorption of thesample concentrated by the virtual impactor.
Ključne besede: dust, black carbon, aerosol
Objavljeno v RUNG: 07.03.2023; Ogledov: 1248; Prenosov: 0
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15. Two-year-long high-time-resolution apportionment of primary and secondary carbonaceous aerosols in the Los Angeles Basin using an advanced total carbon–black carbon (TC-BC([lambda])) methodMatic Ivančič, Asta Gregorič, Gašper Lavrič Palancsai, Bálint Alföldy, Irena Ježek, Sina Hasheminassab, Payam Pakbin, Faraz Ahangar, Mohammad Sowlat, Steven Boddeker, Martin Rigler, 2022, izvirni znanstveni članek Ključne besede: carbonaceous aerosols, black carbon, brown carbon, Carbonaceous Aerosol Speciation System
Objavljeno v RUNG: 04.08.2022; Ogledov: 1392; Prenosov: 8
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18. A dual-wavelength photothermal aerosol absorption monitor : design, calibration and performanceLuka Drinovec, Uroš Jagodič, Luka Pirker, Miha Škarabot, Mario Kurtjak, Kristijan Vidović, Luca Ferrero, Bradley Visser, Jannis Röhrbein, Ernest Weingartner, Daniel M. Kalbermatter, Konstantina Vasilatou, Griša Močnik, 2022, izvirni znanstveni članek Opis: There exists a lack of aerosol absorption measurement techniques with low uncertainties and without artefacts. We have developed the two-wavelength Photothermal Aerosol Absorption Monitor (PTAAM-2λ), which measures the aerosol absorption coefficient at 532 and 1064 nm. Here we describe its design, calibration and mode of operation and evaluate its applicability, limits and uncertainties. The 532 nm channel was calibrated with ∼ 1 µmol mol−1 NO2, whereas the 1064 nm channel was calibrated using measured size distribution spectra of nigrosin particles and a Mie calculation. Since the aerosolized nigrosin used for calibration was dry, we determined the imaginary part of the refractive index of nigrosin from the absorbance measurements on solid thin film samples. The obtained refractive index differed considerably from the one determined using aqueous nigrosin solution. PTAAM-2λ has no scattering artefact and features very low uncertainties: 4 % and 6 % for the absorption coefficient at 532 and 1064 nm, respectively, and 9 % for the absorption Ångström exponent. The artefact-free nature of the measurement method allowed us to investigate the artefacts of filter photometers. Both the Aethalometer AE33 and CLAP suffer from cross-sensitivity to scattering – this scattering artefact is most pronounced for particles smaller than 70 nm. We observed a strong dependence of the filter multiple scattering parameter on the particle size in the 100–500 nm range. The results from the winter ambient campaign in Ljubljana showed similar multiple scattering parameter values for ambient aerosols and laboratory experiments. The spectral dependence of this parameter resulted in AE33 reporting the absorption Ångström exponent for different soot samples with values biased 0.23–0.35 higher than the PTAAM-2λ measurement. Photothermal interferometry is a promising method for reference aerosol absorption measurements.
Ključne besede: aerosol absorption, calibration, black carbon
Objavljeno v RUNG: 28.06.2022; Ogledov: 1177; Prenosov: 25
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19. European Aerosol Phenomenology - 8: Harmonised Source Apportionment of Organic Aerosol using 22 Year-long ACSM/AMS DatasetsGang Chen, Francesco Canonaco, Anna Tobler, Griša Močnik, MaríaCruz Minguillón, André Prévôt, 2022, izvirni znanstveni članek Opis: Organic aerosol (OA) is a key component to total submicron particulate matter (PM1), and comprehensive knowledge of OA sources across Europe is crucial to mitigate PM1 levels. Europe has a well-established air quality research infrastructure from which yearlong datasets using 21 aerosol chemical speciation monitors (ACSMs) and 1 aerosol mass spectrometer (AMS) were gathered during 2013-2019. It includes 9 non-urban and 13 urban sites. This study developed a state-of-the-art source apportionment protocol to analyse long-term OA mass spectrum data by applying the most advanced source apportionment strategies (i.e., rolling PMF, ME-2, and bootstrap). This harmonised protocol was followed strictly for all 22 datasets, making the source apportionment results more comparable. In addition, it enables the quantifications of the most common OA components such as hydrocarbon-like OA (HOA), biomass burning OA (BBOA), cooking-like OA (COA), more oxidised-oxygenated OA (MO-OOA), and less oxidised-oxygenated OA (LO-OOA). Other components such as coal combustion OA (CCOA), solid fuel OA (SFOA: mainly mixture of coal and peat combustion), cigarette smoke OA (CSOA), sea salt (mostly inorganic but part of the OA mass spectrum), coffee OA, and ship industry OA could also be separated at a few specific sites. Oxygenated OA (OOA) components make up most of the submicron OA mass (average = 71.1%, range from 43.7 to 100%). Solid fuel combustion-related OA components (i.e., BBOA, CCOA, and SFOA) are still considerable with in total 16.0% yearly contribution to the OA, yet mainly during winter months (21.4%). Overall, this comprehensive protocol works effectively across all sites governed by different sources and generates robust and consistent source apportionment results. Our work presents a comprehensive overview of OA sources in Europe with a unique combination of high time resolution (30-240 minutes) and long-term data coverage (9-36 months), providing essential information to improve/validate air quality, health impact, and climate models.
Ključne besede: air pollution, source apportionment, organic aeroosl, black carbon
Objavljeno v RUNG: 03.06.2022; Ogledov: 1856; Prenosov: 12
Celotno besedilo (4,69 MB)
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20. Siberian Arctic black carbon : gas flaring and wildfire impactOlga B. Popovicheva, Nikolaos Evangeliou, Vasilii O. Kobelev, Marina A. Chichaeva, Konstantinos Eleftheriadis, Asta Gregorič, Nikolay S. Kasimov, 2022, izvirni znanstveni članek Ključne besede: black carbon, Arctic, gas flaring, wildfire
Objavljeno v RUNG: 09.05.2022; Ogledov: 1543; Prenosov: 0
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