1. Mastering the growth of antimonene on ▫$Bi_2Se_3$▫ : strategies and insightsRoberto Flammini, Conor Hogan, Stefano Colonna, Fabio Ronci, Mauro Satta, Marco Papagno, Ziya S. Aliev, Sergey V. Eremeev, Zipporah Rini Benher, Sandra Gardonio, 2025, original scientific article Abstract: Antimonene, the two-dimensional phase of antimony, appears in two distinct allotropes when epitaxially grown on Bi2Se3: the puckered asymmetric washboard (α) and buckled honeycomb (β) bilayer structures. As-deposited antimony films exhibit varying proportions of single α and β structures. We identify the conditions necessary for ordered, pure-phase growth of single to triple β-antimonene bilayers. Additionally, we determine their electronic structure, work function, and characteristic core-level binding energies, offering an explanation for the relatively large chemical shifts observed among the different phases. This study not only establishes a protocol for achieving a single β phase of antimonene but also provides key signatures for distinguishing between the different allotropes using standard spectroscopic and microscopic techniques.
Keywords: density functional theory, electronic band structure, topological insulators, work functions, scanning tunneling microscopy, atomic structure, antimony, angle-resolved photoemission spectroscopy, core level shifts
Published in RUNG: 20.03.2025; Views: 472; Downloads: 7
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4. Single crystal synthesis and surface electronic structure of Bi_{1.993}Cr_{0.007}Se_{3}Sandra Gardonio, Zipporah Rini Benher, Mattia Fanetti, Paolo Moras, Polina M. Sheverdyaeva, Matjaž Valant, 2024, original scientific article Keywords: topological insulators, magnetic atoms, crystal synthesis, formation of clusters, surface electronic structure
Published in RUNG: 21.08.2024; Views: 1412; Downloads: 8
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7. Giant and tunable out-of-plane spin polarization of topological antimonenePolina M. Sheverdyaeva, Conor Hogan, Gustav Bihlmayer, Jun Fujii, Ivana Vobornik, Matteo Jugovac, Asish K. Kundu, Sandra Gardonio, Zipporah Rini Benher, Giovanni di Santo, 2023, original scientific article Keywords: density functional theory, spin-resolved ARPES, electronic structure, topological insulators, 2D materials, antimonene
Published in RUNG: 18.07.2023; Views: 2629; Downloads: 5
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9. Electronic and chemical surface properties of Bi2Se3 derived compoundsZipporah Rini Benher, doctoral dissertation Keywords: Bismuth selenide derived compounds, surface chemical and electronic properties, topological insulators, single crystals, phase separation, inorganic bulk heterostructures, ix
Bridgman method, X-ray powder diffraction, scanning electron microscopy, photoelectron spectroscopy
Published in RUNG: 16.12.2022; Views: 3634; Downloads: 32
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