| Naslov: | Dissecting Mott and charge-density wave dynamics in the photoinduced phase of 1T-TaS[sub]2 |
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| Avtorji: | Simoncig, Alberto (Avtor)
Stupar, Matija (Avtor)
Ressel, Barbara (Avtor)
Saha, Tanusree (Avtor)
Rebernik Ribič, Primož (Avtor)
De Ninno, Giovanni (Avtor) |
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| Datoteke: | Gradivo nima datotek. Gradivo je morda fizično dosegljivo v knjižnici fakultete, zalogo lahko preverite v COBISS-u.  |
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| Jezik: | Angleški jezik |
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| Vrsta gradiva: | Neznano () |
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| Tipologija: | 1.01 - Izvirni znanstveni članek |
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| Organizacija: | UNG - Univerza v Novi Gorici |
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| Opis: | The two-dimensional transition-metal dichalcogenide 1T−TaS2 is a complex material standing out for its puzzling low temperature phase marked by signatures amenable to both Mott-insulating and charge-density wave states. Electronic Mott states, coupled to a lattice, respond to coherent optical excitations via a modulation of the lower (valence) Hubbard band. Such dynamics is driven by strong electron-phonon coupling and typically lasts for tens of picoseconds, mimicking coherent structural distortions. Instead, the response occurring at the much faster timescale, mainly dominated by electronic many-body effects, is still a matter of intense research. By performing time- and angle-resolved photoemission spectroscopy, we investigated the photoinduced phase of 1T−TaS2 and found out that its lower Hubbard band promptly reacts to coherent optical excitations by shifting its binding energy towards a slightly larger value. This process lasts for a time comparable to the optical pump pulse length, mirroring a transient change of the onsite Coulomb repulsion energy (U). Such an observation suggests that the correction to the bare value of U, ascribed to the phonon-mediated screening which slightly opposes the Hubbard repulsion, is lost within an interval of a few tens of femtoseconds and can be understood as a fingerprint of electronic states largely decoupled from the lattice. Additionally, these results enforce the hypothesis, envisaged in the current literature, that the transient photoinduced states belong to a sort of crossover phase instead of an equilibrium metallic one. |
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| Ključne besede: | ultrafast phenomena, time resolved photoemission, strongly correlated systems, transition metal dichalcogenide |
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| Leto izida: | 2021 |
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| Št. strani: | str. 1-7 |
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| Številčenje: | iss. 5, Vol. 103 |
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| COBISS_ID: | 59328771 |
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| UDK: | 53 |
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| ISSN pri članku: | 2469-9950 |
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| URN: | URN:SI:UNG:REP:OCCSHWAX |
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| DOI: | 10.1103/PhysRevB.103.155120 |
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| Število ogledov: | 961 |
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| Število prenosov: | 0 |
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| Metapodatki: |     |
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| Področja: | Gradivo ni uvrščeno v področja. |
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