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Title:
Mastering the growth of antimonene on ▫$Bi_2Se_3$▫ : strategies and insights
Authors:
ID
Flammini, Roberto
(Author)
ID
Hogan, Conor
(Author)
ID
Colonna, Stefano
(Author)
ID
Ronci, Fabio
(Author)
ID
Satta, Mauro
(Author)
ID
Papagno, Marco
(Author)
ID
Aliev, Ziya S.
(Author)
ID
Eremeev, Sergey V.
(Author)
ID
Benher, Zipporah Rini
(Author)
ID
Gardonio, Sandra
(Author)
Files:
https://pubs.aip.org/aip/apr/article/12/1/011336/3340111/Mastering-the-growth-of-antimonene-on-Bi2Se3
011336_1_5.0246306.pdf
(2,71 MB)
MD5: BC8A67E31C25CA0177F278F90972714A
https://pubs.aip.org/aip/apr/article-pdf/doi/10.1063/5.0246306/20446767/011336_1_5.0246306.pdf
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Language:
English
Work type:
Unknown
Typology:
1.01 - Original Scientific Article
Organization:
UNG - University of Nova Gorica
Abstract:
Antimonene, the two-dimensional phase of antimony, appears in two distinct allotropes when epitaxially grown on Bi2Se3: the puckered asymmetric washboard (α) and buckled honeycomb (β) bilayer structures. As-deposited antimony films exhibit varying proportions of single α and β structures. We identify the conditions necessary for ordered, pure-phase growth of single to triple β-antimonene bilayers. Additionally, we determine their electronic structure, work function, and characteristic core-level binding energies, offering an explanation for the relatively large chemical shifts observed among the different phases. This study not only establishes a protocol for achieving a single β phase of antimonene but also provides key signatures for distinguishing between the different allotropes using standard spectroscopic and microscopic techniques.
Keywords:
density functional theory
,
electronic band structure
,
topological insulators
,
work functions
,
scanning tunneling microscopy
,
atomic structure
,
antimony
,
angle-resolved photoemission spectroscopy
,
core level shifts
Publication status:
Published
Publication version:
Version of Record
Publication date:
01.03.2025
Year of publishing:
2025
Number of pages:
str. 011336-1- 011336-9
Numbering:
Vol. 12, issue 1ǂ, [article no.] 011336
PID:
20.500.12556/RUNG-9919
COBISS.SI-ID:
229662211
UDC:
620.1/.2
ISSN on article:
1931-9401
DOI:
10.1063/5.0246306
NUK URN:
URN:SI:UNG:REP:8BW8GCT5
Publication date in RUNG:
20.03.2025
Views:
388
Downloads:
7
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Record is a part of a journal
Title:
Applied physics reviews
Shortened title:
Appl. phys. rev.
Publisher:
American Institute of Physics
ISSN:
1931-9401
COBISS.SI-ID:
522979097
Document is financed by a project
Funder:
ARIS - Slovenian Research and Innovation Agency
Project number:
P2-0412
Name:
Heterogeni procesi na površinah trdnin za trajnostne tehnologije
Licences
License:
CC BY-NC-ND 4.0, Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International
Link:
http://creativecommons.org/licenses/by-nc-nd/4.0/
Description:
The most restrictive Creative Commons license. This only allows people to download and share the work for no commercial gain and for no other purposes.
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