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Naslov: System size dependence in the Zimm-Bragg model : partition function limits, transition temperature and interval Avtorji: ID Badasyan, Artem (Avtor) Datoteke: https://www.mdpi.com/2073-4360/13/12/1985   Jezik: Angleški jezik Vrsta gradiva: Neznano Tipologija: 1.01 - Izvirni znanstveni članek Organizacija: UNG - Univerza v Novi Gorici Opis: Within the recently developed Hamiltonian formulation of the Zimm and Bragg model we re-evaluate several size dependent approximations of model partition function. Our size analysis is based on the comparison of chain length N with the maximal correlation (persistence) length ξ of helical conformation. For the first time we re-derive the partition function of zipper model by taking the limits of the Zimm–Bragg eigenvalues. The critical consideration of applicability boundaries for the single-sequence (zipper) and the long chain approximations has shown a gap in description for the range of experimentally relevant chain lengths of 5–10 persistence lengths ξ. Correction to the helicity degree expression is reported. For the exact partition function we have additionally found, that: at N/ξ ≈ 10 the transition temperature T m reaches its asymptotic behavior of infinite N; the transition interval ∆T needs about a thousand persistence lengths to saturate at its asymptotic, infinite length value. Obtained results not only contribute to the development of the Zimm–Bragg model, but are also relevant for a wide range of Biotechnologies, including the Biosensing applications. Ključne besede: Zimm-Bragg model, helix-coil transition, zipper model Leto izida: 2021 Št. strani: str. 1-11 Številčenje: Vol. 13, iss. 12 PID: 20.500.12556/RUNG-6595  COBISS.SI-ID: 67393795  UDK: 53 ISSN pri članku: 2073-4360 DOI: 10.3390/polym13121985  NUK URN: URN:SI:UNG:REP:CLG5R7QB Datum objave v RUNG: 17.06.2021 Število ogledov: 2067 Število prenosov: 78 Metapodatki:     Citiraj gradivo Navadno besedilo BibTeX EndNote XML EndNote/Refer RIS ABNT ACM Ref AMA APA Chicago 17th Author-Date Harvard IEEE ISO 690 MLA Vancouver : Kopiraj citat

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Gradivo je del revije

Naslov:	Polymers
Skrajšan naslov:	Polymers
Založnik:	Molecular Diversity Preservation International
ISSN:	2073-4360
COBISS.SI-ID:	517951257

Gradivo je financirano iz projekta

Financer:	ARRS - Agencija za raziskovalno dejavnost Republike Slovenije
Številka projekta:	J1-1705; P2-0412

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