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Title:Comparing black-carbon- and aerosol-absorption-measuring instruments – a new system using lab-generated soot coated with controlled amounts of secondary organic matter
Authors:ID Kalbermatter, Daniel M. (Author)
ID Močnik, Griša (Author)
ID Drinovec, Luka (Author)
ID Visser, Bradley (Author)
ID Röhrbein, Jannis (Author)
ID Oscity, Matthias (Author)
ID Weingartner, Ernest (Author)
ID Hyvärinen, Antti-Pekka (Author)
ID Vasilatou, Konstantina (Author)
Files:.pdf Kalbermatter_-_AMT_2022_-_Comparing_BC_and_aerosol-absorption-measuring_instruments_–_a_new_system_using_lab-generated_soot_coated_with_controlled_amounts_of_SOA.pdf (752,94 KB)
MD5: 3182F18945B00370ABAFA97C781172BA
 
Language:English
Work type:Unknown
Typology:1.01 - Original Scientific Article
Organization:UNG - University of Nova Gorica
Abstract:We report on an inter-comparison of black-carbon- and aerosol-absorption-measuring instruments with laboratory-generated soot particles coated with controlled amounts of secondary organic matter (SOM). The aerosol generation setup consisted of a miniCAST 5201 Type BC burner for the generation of soot particles and a new automated oxidation flow reactor based on the micro smog chamber (MSC) for the generation of SOM from the ozonolysis of α-pinene. A series of test aerosols was generated with elemental to total carbon (EC  TC) mass fraction ranging from about 90 % down to 10 % and single-scattering albedo (SSA at 637 nm) from almost 0 to about 0.7. A dual-spot Aethalometer AE33, a photoacoustic extinctiometer (PAX, 870 nm), a multi-angle absorption photometer (MAAP), a prototype photoacoustic instrument, and two prototype photo-thermal interferometers (PTAAM-2λ and MSPTI) were exposed to the test aerosols in parallel. Significant deviations in the response of the instruments were observed depending on the amount of secondary organic coating. We believe that the setup and methodology described in this study can easily be standardised and provide a straightforward and reproducible procedure for the inter-comparison and characterisation of both filter-based and in situ black-carbon-measuring (BC-measuring) instruments based on realistic test aerosols.
Keywords:black carbon, aerosol absorption, secondary organic aerosol, coating
Year of publishing:2022
Number of pages:str. 561-572
Numbering:Vol. 15, iss. 2
PID:20.500.12556/RUNG-7164 New window
COBISS.SI-ID:95895811 New window
UDC:502.3/.7
ISSN on article:1867-8548
DOI:10.5194/amt-15-561-2022 New window
NUK URN:URN:SI:UNG:REP:UGUFQOPD
Publication date in RUNG:01.02.2022
Views:1611
Downloads:48
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Record is a part of a journal

Title:Atmospheric measurement techniques
Shortened title:Atmos. meas. tech.
Publisher:Copernicus Publications
ISSN:1867-8548
COBISS.SI-ID:522351897 New window

Licences

License:CC BY 4.0, Creative Commons Attribution 4.0 International
Link:http://creativecommons.org/licenses/by/4.0/
Description:This is the standard Creative Commons license that gives others maximum freedom to do what they want with the work as long as they credit the author.
Licensing start date:01.02.2022

Secondary language

Language:Undetermined
Title:Comparing black-carbon- and aerosol-absorption-measuring instruments


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