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Title:European Aerosol Phenomenology - 8: Harmonised Source Apportionment of Organic Aerosol using 22 Year-long ACSM/AMS Datasets
Authors:ID Chen, Gang, Paul Scherrer Institut (Author)
ID Canonaco, Francesco, Datalystica (Author)
ID Tobler, Anna, Datalystica (Author)
ID Močnik, Griša, University of Nova Gorica (Author)
ID Minguillón, MaríaCruz, IDAEA-CSIC (Author)
ID Prévôt, André, Paul Scherrer Institut (Author), et al.
Files:.pdf Chen_-_EI_2022_-_European_Aerosol_Phenomenology_8-_Harmonised_Source_Apportionment_of_Organic_Aerosol_using_22_Year-long_ACSM_AMS_Datasets.pdf (4,69 MB)
MD5: EC2916BFE5047732000152D8325CFFA6
.pdf RAZ_Chen_Gang_i2022.pdf (6,37 MB)
MD5: E63865321BFC6AD064C50FD895357AA7
Work type:Not categorized
Typology:1.01 - Original Scientific Article
Organization:UNG - University of Nova Gorica
Abstract:Organic aerosol (OA) is a key component to total submicron particulate matter (PM1), and comprehensive knowledge of OA sources across Europe is crucial to mitigate PM1 levels. Europe has a well-established air quality research infrastructure from which yearlong datasets using 21 aerosol chemical speciation monitors (ACSMs) and 1 aerosol mass spectrometer (AMS) were gathered during 2013-2019. It includes 9 non-urban and 13 urban sites. This study developed a state-of-the-art source apportionment protocol to analyse long-term OA mass spectrum data by applying the most advanced source apportionment strategies (i.e., rolling PMF, ME-2, and bootstrap). This harmonised protocol was followed strictly for all 22 datasets, making the source apportionment results more comparable. In addition, it enables the quantifications of the most common OA components such as hydrocarbon-like OA (HOA), biomass burning OA (BBOA), cooking-like OA (COA), more oxidised-oxygenated OA (MO-OOA), and less oxidised-oxygenated OA (LO-OOA). Other components such as coal combustion OA (CCOA), solid fuel OA (SFOA: mainly mixture of coal and peat combustion), cigarette smoke OA (CSOA), sea salt (mostly inorganic but part of the OA mass spectrum), coffee OA, and ship industry OA could also be separated at a few specific sites. Oxygenated OA (OOA) components make up most of the submicron OA mass (average = 71.1%, range from 43.7 to 100%). Solid fuel combustion-related OA components (i.e., BBOA, CCOA, and SFOA) are still considerable with in total 16.0% yearly contribution to the OA, yet mainly during winter months (21.4%). Overall, this comprehensive protocol works effectively across all sites governed by different sources and generates robust and consistent source apportionment results. Our work presents a comprehensive overview of OA sources in Europe with a unique combination of high time resolution (30-240 minutes) and long-term data coverage (9-36 months), providing essential information to improve/validate air quality, health impact, and climate models.
Keywords:air pollution, source apportionment, organic aeroosl, black carbon
Publication version:Author Accepted Manuscript
Year of publishing:2022
Number of pages:63
PID:20.500.12556/RUNG-7359 New window
COBISS.SI-ID:110392067 New window
DOI:10.1016/j.envint.2022.107325 New window
Publication date in RUNG:03.06.2022
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Record is a part of a journal

Title:Environment International
Shortened title:Environ. Int.
Year of publishing:2022

Document is financed by a project

Funder:ARRS - Agencija za raziskovalno dejavnost Republike Slovenije
Project number:P1- 0385
Name:Daljinsko zaznavanje atmosferskih lastnosti


License:CC BY-SA 4.0, Creative Commons Attribution-ShareAlike 4.0 International
Description:This Creative Commons license is very similar to the regular Attribution license, but requires the release of all derivative works under this same license.
Licensing start date:03.06.2022